Lithium-ion (Li-ion) batteries have become the leading energy storage technology, powering a wide range of applications in today's electrified world. This comprehensive review paper delves into the current challenges and innovative solutions driving the supercharged future of lithium-ion batteries. It scrutinizes the limitations of energy density in existing batteries, exploring advanced electrode materials and designs that promise higher capacity. Safety concerns take center stage, with a focus on cutting-edge thermal management systems and materials. The imperative of sustainable sourcing is addressed, highlighting alternative materials and recycling strategies for a greener supply chain. Transformative breakthroughs, such as solid-state electrolytes and emerging battery chemistries, offer glimpses of the future. The paper also examines the applications and market perspectives of lithium-ion batteries in electric vehicles, portable electronics, and renewable energy storage. It concludes by emphasizing the transformative potential of lithium-ion batteries in accelerating the energy revolution and paving the way for a sustainable energy future.

Revolutionizing energy storage: Overcoming challenges and unleashing the potential of next generation Lithium-ion battery technology

With the successive retirement of lithium-ion batteries (LIBs) approaching, there has been an upsurge of spent LIBs, posing significant challenges to energy, resources, and environment, which has led to the...

A systematic review of efficient recycling for cathode materials of spent lithium-ion batteries: process intensification technologies beyond traditional methods

A large deal of knowledge about recycling offers hope for the future in this day and age when trash resulting from several systems or items is a major concern. This article compiles and presents to the readers the most recent research on the recycling of active elements in Li-ion batteries, the widely used energy storage devices in recent years. At this stage, as a critical examination of the literature, current techniques and procedures for recycling frequently used Li-ion battery types, including LCO, LFP, LMO, NMC, and NCA batteries, are discussed. In general, data on the recycling effectiveness of the three types of recycling processes—pyrometallurgy, hydrometallurgy, and mechanical separation—as well as any reuse of recovered materials have been collated and presented. It is intended that this review article would aid readers' studies and researches because the significance of recycling used Li-ion batteries is growing every day. 

Recycling valuable materials from the cathodes of spent lithium-ion batteries: A comprehensive review

All-solid state lithium metal batteries (ASSLMBs) with high energy density using lithium metal anodes (LMAs) and high safety all-solid-state electrolytes (ASSEs) are considered as a good choice for the next...

Strategies to regulate the interface between Li metal anode and all-solid-state electrolyte

The overall crushing of spent ternary lithium-ion batteries (SNCM) makes the mix of the anode and cathode electrode materials. Multiple separation not only wastes energy, causes secondary pollution but also fails to achieve the excellent separation of the valuable component. Therefore, this paper reviewed the recycling methods of SNCM from three aspects, including the single recycling of anode, the single recycling of cathode electrode materials and the overall collaborative recycling of anode and cathode electrode materials. The necessity of high-purity separation of the anode and cathode electrode materials was discussed by evaluating the difference between single recycling and overall collaborative recycling. A process that used collaborative reclaim to realize efficient and green resource utilization of electrode materials was proposed based on the review. In this process, the mixed electrode materials were first divided into rich cathode-poor anode materials and rich anode-poor cathode materials by flotation. Two kinds of materials were regenerated to prepare NCM. The recovery of the cathode was enhanced through the reduction properties of the anode. The electrochemical properties of the regenerated anode were enhanced by the in-situ self-utilization behavior of the cathode. The recovery process was optimized by simplifying the process and improving efficiency. The economic and green of the recovery process was ensured by treating the SNCM with readily available and environmentally friendly agents. 

Review on the sustainable recycling of spent ternary lithium-ion batteries: From an eco-friendly and efficient perspective

Solid-state electrolytes attract great attention due to their advantages in safety, electrochemical stability and battery packaging. High-voltage cathode materials and the Li metal anode further increase the energy density and electrochemical cycling properties.

A review of all-solid-state electrolytes for lithium batteries: high-voltage cathode materials, solid-state electrolytes and electrode–electrolyte interfaces

Recovered Cobalt-Nickel Sulfide from spent lithium-ion batteries as an advanced anode material toward sodium-ion batteries

Ultrahigh salt content enables the nonflammable PVDF-based solid electrolyte with high ionic conductivity

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A review of all-solid-state electrolytes for lithium batteries: high-voltage cathode materials, solid-state electrolytes and electrode–electrolyte interfaces

Recovered Cobalt-Nickel Sulfide from spent lithium-ion batteries as an advanced anode material toward sodium-ion batteries

Ultrahigh salt content enables the nonflammable PVDF-based solid electrolyte with high ionic conductivity