The development of efficient and affordable electrode materials is crucial for clean energy storage systems, which are considered a promising strategy for addressing energy crises and environmental issues. Metal phosphorous chalcogenides (MPX3 ) are a fascinating class of two-dimensional materials with a tunable layered structure and high ion conductivity, making them particularly attractive for energy storage applications. This review article aims to comprehensively summarize the latest research progress on MPX3 materials, with a focus on their preparation methods and modulation strategies. Additionally, the diverse applications of these novel materials in alkali metal ion batteries, metal-air batteries, and all-solid-state batteries are highlighted. Finally, the challenges and opportunities of MPX3 materials are presented to inspire their better potential in energy storage applications. This review provides valuable insights into the promising future of MPX3 materials in clean energy storage systems. 

Metal Phosphorous Chalcogenide: A Promising Material for Advanced Energy Storage Systems.

The exploration of high-energy density flexible electrodes through reasonable structural design is the key to realizing the overall portability and wearability of devices. Herein, a free-standing hybrid nanofabric with superior mechanical and electrochemical stabilities is reported for flexible lithium-ion batteries (LIBs). The hybrid nanofabric is prepared by electrospinning and carbonization, during which the self-cyclization of polyacrylonitrile (PAN) is hindered by its reaction with melamine, resulting in a highly disordered and expanded turbostratic carbon structure with nickel metal thiophosphate (NiPS3) nanosheets embedded in it. The coordinated movement of the electrospun-derived 1D nanofiber, the super toughness of the hard carbon structure and the interlayer slipping of NiPS3 endow the hybrid nanofabric with excellent tolerance to large-scale deformation. It can be folded three times in half and quickly return to its original state. When used as the anode for LIBs, no additional binder, conducting agent and current collector are needed. The free-standing anode not only shows excellent cycling (797.5 mA h g-1 after 1000 cycles at 1 A g-1) and rate (more than 56% capacity retained from 0.1 to 2 A g-1) performances, but also maintains its original electrochemical properties after being folded 300 times at 120°, 180° and 360°. This work provides a synergistic strategy to simultaneously enhance the energy density and flexibility of a fabric electrode, paving the way for the application of advanced flexible energy storage systems.

Realizing the high energy density and flexibility of a fabric electrode through hierarchical structure design.

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Between the State and the Society: the Path Selection of Response to Extreme Climate in Ancient China

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Realizing the high energy density and flexibility of a fabric electrode through hierarchical structure design.

Between the State and the Society: the Path Selection of Response to Extreme Climate in Ancient China