TL;DR: In this paper, the results of a series of experiments in which a giant pulsed ruby laser is used to study several different nonlinear optical effects arising from an induced optical polarization third order in the electric field strength are presented.
Abstract: This paper presents the results of a series of experiments in which a giant pulsed ruby laser is used to study several different nonlinear optical effects arising from an induced optical polarization third order in the electric field strength. The various phenomena studied are special cases of either frequency mixing or intensity-dependent changes in the complex refractive index, including Raman laser action at a focus. A wide range of crystalline and isotropic materials was studied. The theory for these effects is extended to cover resonant interactions. The experimental results are interpreted in terms of simplified models, and quantitative values for the nonlinear polarizability coefficients are given. The rather large experimental uncertainties in these coefficients are discussed.
TL;DR: In this article, a quantum mechanical model for parametric interactions is used to evaluate the effect of the measuring (amplifying) process on the statistical properties of radiation, and it is shown that it allows a simultaneous determination of the phase and number of quanta of an electromagnetic wave with an accuracy which is limited only by the uncertainty principle.
Abstract: A quantum mechanical model for parametric interactions is used to evaluate the effect of the measuring (amplifying) process on the statistical properties of radiation. Parametric amplification is shown to be ideal in the sense that it allows a simultaneous determination of the phase and number of quanta of an electromagnetic wave with an accuracy which is limited only by the uncertainty principle. Frequency conversion via parametric processes is shown to be free of zero-point fluctuations.
TL;DR: The quantum state of optical pulses containing single photons is reconstructed using the method of phase-randomized pulsed optical homodyne tomography and shows a strong dip reaching classically impossible negative values around the origin of the phase space.
Abstract: We have reconstructed the quantum state of optical pulses containing single photons using the method of phase-randomized pulsed optical homodyne tomography. The single-photon Fock state 1> was prepared using conditional measurements on photon pairs born in the process of parametric down-conversion. A probability distribution of the phase-averaged electric field amplitudes with a strongly non-Gaussian shape is obtained with the total detection efficiency of (55+/-1)%. The angle-averaged Wigner function reconstructed from this distribution shows a strong dip reaching classically impossible negative values around the origin of the phase space.
TL;DR: The ultrafast reversibility of the effects implies that the physical properties of a dielectric can be controlled with the electric field of light, offering the potential for petahertz-bandwidth signal manipulation.
Abstract: The ultrafast reversibility of changes to the electronic structure and electric polarizability of a dielectric with the electric field of a laser pulse, demonstrated here, offers the potential for petahertz-bandwidth optical signal manipulation. Two studies published in this issue highlight the potential for ultrafast signal manipulation in dielectrics using optical fields. When it comes to electrical signal processing, semiconductors have become the materials of choice. However, insulators such as dielectrics could be attractive alternatives: they have a fast response in principle, but usually have extremely low conductivity at low electric fields and break down in large fields. The electronic properties of dielectrics can be controlled with few-cycle laser pulses that permit damage-free exposure of dielectrics to high electric fields. Agustin Schiffrin et al. demonstrate that strong optical laser fields with controlled few-cycle waveforms can reversibly transform a dielectric insulator into a conductor within the optical period (within one femtosecond). Martin Schultze et al. address the crucial issue of ultrafast reversibility, demonstrating that the dielectric can be repeatedly switched 'on' and 'off' with light fields, without degradation. The control of the electric and optical properties of semiconductors with microwave fields forms the basis of modern electronics, information processing and optical communications. The extension of such control to optical frequencies calls for wideband materials such as dielectrics, which require strong electric fields to alter their physical properties1,2,3,4,5. Few-cycle laser pulses permit damage-free exposure of dielectrics to electric fields of several volts per angstrom6 and significant modifications in their electronic system6,7,8,9,10,11,12,13. Fields of such strength and temporal confinement can turn a dielectric from an insulating state to a conducting state within the optical period14. However, to extend electric signal control and processing to light frequencies depends on the feasibility of reversing these effects approximately as fast as they can be induced. Here we study the underlying electron processes with sub-femtosecond solid-state spectroscopy, which reveals the feasibility of manipulating the electronic structure and electric polarizability of a dielectric reversibly with the electric field of light. We irradiate a dielectric (fused silica) with a waveform-controlled near-infrared few-cycle light field of several volts per angstrom and probe changes in extreme-ultraviolet absorptivity and near-infrared reflectivity on a timescale of approximately a hundred attoseconds to a few femtoseconds. The field-induced changes follow, in a highly nonlinear fashion, the turn-on and turn-off behaviour of the driving field, in agreement with the predictions of a quantum mechanical model. The ultrafast reversibility of the effects implies that the physical properties of a dielectric can be controlled with the electric field of light, offering the potential for petahertz-bandwidth signal manipulation.
TL;DR: A frequency comb spanning an octave via the parametric process of cascaded four-wave mixing in a monolithic, high-Q silicon nitride microring resonator is demonstrated and it is found that the comb can operate in a low-noise state with a 30 dB reduction in noise as the pump frequency is tuned into the cavity resonance.
Abstract: We demonstrate a frequency comb spanning an octave via the parametric process of cascaded four-wave mixing in a monolithic, high-Q silicon nitride microring resonator. The comb is generated from a single-frequency pump laser at 1562 nm and spans 128 THz with a spacing of 226 GHz, which can be tuned slightly with the pump power. In addition, we investigate the RF-noise characteristics of the parametric comb and find that the comb can operate in a low-noise state with a 30-dB reduction in noise as the pump frequency is tuned into the cavity resonance.