TL;DR: In this article, the optical properties of aerosols and clouds are described, including extinction, scattering, and absorption coefficients, single scattering albedo, asymmetry parameter, and phase function.
Abstract: The software package OPAC (Optical Properties of Aerosols and Clouds) is described. It easily provides optical properties in the solar and terrestrial spectral range of atmospheric particulate matter. Microphysical and optical properties of six water clouds, three ice clouds, and 10 aerosol components, which are considered as typical cases, are stored as ASCII files. The optical properties are the extinction, scattering, and absorption coefficients, the single scattering albedo, the asymmetry parameter, and the phase function. They are calculated on the basis of the microphysical data (size distribution and spectral refractive index) under the assumption of spherical particles in case of aerosols and cloud droplets and assuming hexagonal columns in case of cirrus clouds. Data are given for up to 61 wavelengths between 0.25 and 40 μm and up to eight values of the relative humidity. The software package also allows calculation of derived optical properties like mass extinction coefficients and Angstrom coefficients. Real aerosol in the atmosphere always is a mixture of different components. Thus, in OPAC it is made possible to get optical properties of any mixtures of the basic components and to calculate optical depths on the base of exponential aerosol height profiles. Typical mixtures of aerosol components as well as typical height profiles are proposed as default values, but mixtures and profiles for the description of individual cases may also be achieved simply.
TL;DR: In this paper, a revised approach to cloud microphysical processes in a commonly used bulk microphysics parameterization and the importance of correctly representing properties of cloud ice are discussed, and the impact of sedimentation of ice crystals is also investigated.
Abstract: A revised approach to cloud microphysical processes in a commonly used bulk microphysics parameterization and the importance of correctly representing properties of cloud ice are discussed. Several modifications are introduced to more realistically simulate some of the ice microphysical processes. In addition to the assumption that ice nuclei number concentration is a function of temperature, a new and separate assumption is developed in which ice crystal number concentration is a function of ice amount. Related changes in ice microphysics are introduced, and the impact of sedimentation of ice crystals is also investigated. In an idealized thunderstorm simulation, the distribution of simulated clouds and precipitation is sensitive to the assumptions in microphysical processes, whereas the impact of the sedimentation of cloud ice is small. Overall, the modifications introduced to microphysical processes play a role in significantly reducing cloud ice and increasing snow at colder temperatures and ...
TL;DR: A two-moment cloud microphysics scheme predicting the mixing ratios and number concentrations of five species (i.e., cloud droplets, cloud ice, snow, rain, and graupel) has been implemented into the Weather Research and Forecasting model (WRF) as discussed by the authors.
Abstract: A new two-moment cloud microphysics scheme predicting the mixing ratios and number concentrations of five species (i.e., cloud droplets, cloud ice, snow, rain, and graupel) has been implemented into the Weather Research and Forecasting model (WRF). This scheme is used to investigate the formation and evolution of trailing stratiform precipitation in an idealized two-dimensional squall line. Results are compared to those using a one-moment version of the scheme that predicts only the mixing ratios of the species, and diagnoses the number concentrations from the specified size distribution intercept parameter and predicted mixing ratio. The overall structure of the storm is similar using either the one- or two-moment schemes, although there are notable differences. The two-moment (2-M) scheme produces a widespread region of trailing stratiform precipitation within several hours of the storm formation. In contrast, there is negligible trailing stratiform precipitation using the one-moment (1-M) scheme. The primary reason for this difference are reduced rain evaporation rates in 2-M compared to 1-M in the trailing stratiform region, leading directly to greater rain mixing ratios and surface rainfall rates. Second, increased rain evaporation rates in 2-M compared to 1-M in the convective region at midlevels result in weaker convective updraft cells and increased midlevel detrainment and flux of positively buoyant air from the convective into the stratiform region. This flux is in turn associated with a stronger mesoscale updraft in the stratiform region and enhanced ice growth rates. The reduced (increased) rates of rain evaporation in the stratiform (convective) regions in 2-M are associated with differences in the predicted rain size distribution intercept parameter (which was specified as a constant in 1-M) between the two regions. This variability is consistent with surface disdrometer measurements in previous studies that show a rapid decrease of the rain intercept parameter during the transition from convective to stratiform rainfall.
TL;DR: Zhang et al. as discussed by the authors used a more advanced NASA Goddard Institute for Space Studies (GISS) radiative transfer model and improved ISCCP cloud climatology and ancillary data sets.
Abstract: [1] We continue reconstructing Earth’s radiation budget from global observations in as much detail as possible to allow diagnosis of the effects of cloud (and surface and other atmospheric constituents) variations on it. This new study was undertaken to reduce the most noticeable systematic errors in our previous results (flux data set calculated mainly using International Satellite Cloud Climatology Project–C1 input data (ISCCP-FC)) by exploiting the availability of a more advanced NASA Goddard Institute for Space Studies (GISS) radiative transfer model and improved ISCCP cloud climatology and ancillary data sets. The most important changes are the introduction of a better treatment of ice clouds, revision of the aerosol climatology, accounting for diurnal variations of surface skin/air temperatures and the cloud-radiative effects on them, revision of the water vapor profiles used, and refinement of the land surface albedos and emissivities. We also extend our previous flux results, limited to the top of atmosphere (TOA) and surface (SRF), to also include three levels within the atmosphere, forming one integrated vertical atmospheric flux profile from SRF to TOA, inclusive, by combining a new climatology of cloud vertical structure with the ISCCP cloud product. Using the new radiative transfer model and new input data sets, we have produced an 18-year at 3-hour time steps, global at 280-km intervals, radiative flux profile data set (called ISCCP-FD) that provides full- and clear-sky, shortwave and longwave, upwelling and downwelling fluxes at five levels (SRF, 680 mbar, 440 mbar, 100 mbar, and TOA). Evaluation is still only possible for TOA and SRF fluxes: Comparisons of monthly, regional mean values from FD with Earth Radiation Budget Experiment, Clouds and the Earth’s Radiant Energy System and Baseline Surface Radiation Network values suggest that we have been able to reduce the overall uncertainties from 10–15 to 5–10 W/m 2 at TOA and from 20–25 to 10– 15 W/m 2 at SRF. Annual mean pressure-latitude cross sections of the cloud effects on atmospheric net radiative fluxes show that clouds shift the longwave cooling downward in the Intertropical Convergence Zone, acting to stabilize the tropical atmosphere while increasing the horizontal heating gradient forcing the Hadley circulation, and shift the longwave cooling upward in the midlatitude storm zones, acting to destabilize the baroclinic zones while decreasing the horizontal heating gradient there. INDEX TERMS: 1620 Global Change: Climate dynamics (3309); 3309 Meteorology and Atmospheric Dynamics: Climatology (1620); 3359 Meteorology and Atmospheric Dynamics: Radiative processes; KEYWORDS: Earth radiation budget, surface radiation budget (SRB), cloud vertical structure, ERBE, CERES, BSRN Citation: Zhang, Y., W. B. Rossow, A. A. Lacis, V. Oinas, and M. I. Mishchenko (2004), Calculation of radiative fluxes from the surface to top of atmosphere based on ISCCP and other global data sets: Refinements of the radiative transfer model and the input data, J. Geophys. Res., 109, D19105, doi:10.1029/2003JD004457.
TL;DR: In this paper, a double-moment bulk microphysics scheme predicting the number concentrations and mixing ratios of four hydrometeor species (droplets, cloud ice, rain, snow) is described.
Abstract: A new double-moment bulk microphysics scheme predicting the number concentrations and mixing ratios of four hydrometeor species (droplets, cloud ice, rain, snow) is described. New physically based parameterizations are developed for simulating homogeneous and heterogeneous ice nucleation, droplet activation, and the spectral index (width) of the droplet size spectra. Two versions of the scheme are described: one for application in high-resolution cloud models and the other for simulating grid-scale cloudiness in larger-scale models. The versions differ in their treatment of the supersaturation field and droplet nucleation. For the high-resolution approach, droplet nucleation is calculated from Kohler theory applied to a distribution of aerosol that activates at a given supersaturation. The resolved supersaturation field and condensation/deposition rates are predicted using a semianalytic approximation to the three-phase (vapor, ice, liquid) supersaturation equation. For the large-scale version of the scheme, it is assumed that the supersaturation field is not resolved and thus droplet activation is parameterized as a function of the vertical velocity and diabatic cooling rate. The vertical velocity includes a subgrid component that is parameterized in terms of the eddy diffusivity and mixing length. Droplet condensation is calculated using a quasi-steady, saturation adjustment approach. Evaporation/deposition onto the other water species is given by nonsteady vapor diffusion allowing excess vapor density relative to ice saturation.