TL;DR: In this paper, the photodissociation processes occurring in molecular oxygen following the two-photon 3dπ(3Σ1g −) Rydberg excitation around 225 nm are presented to show the improvement in spatial resolution in the ion and electron images.
Abstract: The application of electrostatic lenses is demonstrated to give a substantial improvement of the two-dimensional (2D) ion/electron imaging technique. This combination of ion lens optics and 2D detection makes “velocity map imaging” possible, i.e., all particles with the same initial velocity vector are mapped onto the same point on the detector. Whereas the more common application of grid electrodes leads to transmission reduction, severe trajectory deflections and blurring due to the non-point source geometry, these problems are avoided with open lens electrodes. A three-plate assembly with aperture electrodes has been tested and its properties are compared with those of grid electrodes. The photodissociation processes occurring in molecular oxygen following the two-photon 3dπ(3Σ1g −)(v=2, N=2)←X(3Σg −) Rydberg excitation around 225 nm are presented here to show the improvement in spatial resolution in the ion and electron images. Simulated trajectory calculations show good agreement with experiment and ...
TL;DR: In this article, the authors reported the observation of conductance oscillations in extremely narrow graphene heterostructures where a resonant cavity is formed between two electrostatically created bipolar junctions.
Abstract: The observation of oscillations in the conductance characteristics of narrow graphene p–n-junctions confirms their ability to collimate ballistic carriers. Moreover, the phase of these oscillations at low magnetic field suggests the occurrence of the perfect transmission of carriers normal to the junction as a direct result of the Klein effect. The observation of quantum conductance oscillations in mesoscopic systems has traditionally required the confinement of the carriers to a phase space of reduced dimensionality1,2,3,4. Although electron optics such as lensing5 and focusing6 have been demonstrated experimentally, building a collimated electron interferometer in two unconfined dimensions has remained a challenge owing to the difficulty of creating electrostatic barriers that are sharp on the order of the electron wavelength7. Here, we report the observation of conductance oscillations in extremely narrow graphene heterostructures where a resonant cavity is formed between two electrostatically created bipolar junctions. Analysis of the oscillations confirms that p–n junctions have a collimating effect on ballistically transmitted carriers8. The phase shift observed in the conductance fringes at low magnetic fields is a signature of the perfect transmission of carriers normally incident on the junctions9 and thus constitutes a direct experimental observation of ‘Klein tunnelling’10,11,12.
TL;DR: The focusing of electric current by a single p-n junction in graphene is theoretically predicted and may be useful for the engineering of electronic lenses and focused beam splitters using gate-controlled n-p-n junctions in graphene-based transistors.
Abstract: The focusing of electric current by a single p-n junction in graphene is theoretically predicted. Precise focusing may be achieved by fine-tuning the densities of carriers on the n- and p-sides of the junction to equal values. This finding may be useful for the engineering of electronic lenses and focused beam splitters using gate-controlled n-p-n junctions in graphene-based transistors.
TL;DR: This technique is a reproducible method of creating vortex electron beams in a conventional electron microscope, and it is demonstrated how they may be used in electron energy-loss spectroscopy to detect the magnetic state of materials and describe their properties.
Abstract: It has been possible to produce photon vortex beams — optical beams with spiralling wavefronts — for some time, and they have found widespread application as optical tweezers, in interferometry and in information transfer, for example. The production of vortex beams of electrons was demonstrated earlier this year (
http://go.nature.com/4H2xWR
) in a procedure involving the passage of electrons through a spiral stack of graphite thin films. The ability to generate such beams reproducibly in a conventional electron microscope would enable many new applications. Now Jo Verbeeck and colleagues have taken a step towards that goal. They describe a versatile holographic technique for generating these twisted electron beams, and demonstrate their potential use as probes of a material's magnetic properties. It was demonstrated recently that passing electrons through a spiral stack of graphite thin films generates an electron beam with orbital angular momentum — analogous to the spiralling wavefronts that can be introduced in photon beams and which have found widespread application. Here, a versatile holographic technique for generating these twisted electron beams is described. Moreover, a demonstration is provided of their potential use in probing a material's magnetic properties. Vortex beams (also known as beams with a phase singularity) consist of spiralling wavefronts that give rise to angular momentum around the propagation direction. Vortex photon beams are widely used in applications such as optical tweezers to manipulate micrometre-sized particles and in micro-motors to provide angular momentum1,2, improving channel capacity in optical3 and radio-wave4 information transfer, astrophysics5 and so on6. Very recently, an experimental realization of vortex beams formed of electrons was demonstrated7. Here we describe the creation of vortex electron beams, making use of a versatile holographic reconstruction technique in a transmission electron microscope. This technique is a reproducible method of creating vortex electron beams in a conventional electron microscope. We demonstrate how they may be used in electron energy-loss spectroscopy to detect the magnetic state of materials and describe their properties. Our results show that electron vortex beams hold promise for new applications, in particular for analysing and manipulating nanomaterials, and can be easily produced.
TL;DR: The implementation of a computer-controlled aberration correction system in a scanning transmission electron microscope, which is less sensitive to chromatic aberration, is reported here and allows dynamic imaging of single atoms, clusters of a few atoms, and single atomic layer ‘rafts' of atoms coexisting with Au islands on a carbon substrate.
Abstract: Following the invention of electron optics during the 1930s, lens aberrations have limited the achievable spatial resolution to about 50 times the wavelength of the imaging electrons. This situation is similar to that faced by Leeuwenhoek in the seventeenth century, whose work to improve the quality of glass lenses led directly to his discovery of the ubiquitous "animalcules" in canal water, the first hints of the cellular basis of life. The electron optical aberration problem was well understood from the start, but more than 60 years elapsed before a practical correction scheme for electron microscopy was demonstrated, and even then the remaining chromatic aberrations still limited the resolution. We report here the implementation of a computer-controlled aberration correction system in a scanning transmission electron microscope, which is less sensitive to chromatic aberration. Using this approach, we achieve an electron probe smaller than 1 A. This performance, about 20 times the electron wavelength at 120 keV energy, allows dynamic imaging of single atoms, clusters of a few atoms, and single atomic layer 'rafts' of atoms coexisting with Au islands on a carbon substrate. This technique should also allow atomic column imaging of semiconductors, for detection of single dopant atoms, using an electron beam with energy below the damage threshold for silicon.