TL;DR: It is shown that for the worst cases of severe range dependence in aerosol backscattering, the residual errors in the corrected DIAL O3 measurements were <10 ppbv for DIAL wavelengths at 286 and 300 nm.
Abstract: The differential absorption lidar (DIAL) technique generally assumes that atmospheric optical scattering is the same at the two laser wavelengths used in the DIAL measurement of a gas concentration profile. Errors can arise in this approach when the wavelengths are significantly separated, and there is a range dependence in the aerosol scattering distribution. This paper discusses the errors introduced by large DIAL wavelength separations and spatial inhomogeneity of aerosols in the atmosphere. A Bernoulli solution for determining the relative distribution of aerosol backscattering in the UV region is presented, and scattering ratio boundary values for these solutions are discussed. The results of this approach are used to derive a backscatter correction to the standard DIAL analysis method. It is shown that for the worst cases of severe range dependence in aerosol backscattering, the residual errors in the corrected DIAL O3 measurements were <10 ppbv for DIAL wavelengths at 286 and 300 nm.
TL;DR: In this paper, a Bernoulli solution for determining the relative distribution of aerosol backscattering in the UV region is presented, and scattering ratio boundary values for these solutions are discussed.
Abstract: The differential absorption lidar (DIAL) technique generally assumes that atmospheric optical scattering is the same at the two laser wavelengths used in the DIAL measurement of a gas concentration profile. Errors can arise in this approach when the wavelengths are significantly separated, and there is a range dependence in the aerosol scattering distribution. This paper discusses the errors introduced by large DIAL wavelength separations and spatial inhomogeneity of aerosols in the atmosphere. A Bernoulli solution for determining the relative distribution of aerosol backscattering in the UV region is presented, and scattering ratio boundary values for these solutions are discussed. The results of this approach are used to derive a backscatter correction to the standard DIAL analysis method. It is shown that for the worst cases of severe range dependence in aerosol backscattering, the residual errors in the corrected DIAL O3 measurements were <10 ppbv for DIAL wavelengths at 286 and 300 nm.
TL;DR: The NASA airborne differential absorption lidar (DIAL) system as discussed by the authors was designed to assess the average gas concentration over a specified range interval by analyzing the difference in lidar backscatter signals for laser wavelengths tuned on and off of the molecular absorption line of a gas under investigation.
Abstract: The hardware, operational characteristics, data processing system, and applications of the NASA airborne differential absorption lidar (DIAL) system are described. DIAL functions by assessing the average gas concentration over a specified range interval by analyzing the difference in lidar backscatter signals for laser wavelengths tuned on and off of the molecular absorption line of a gas under investigation. The system comprises two frequency-doubled Nd:YAG lasers pumping two high conversion efficiency tunable dye lasers emitting pulses separated by 100 microsec or less. The return signals are digitized and stored on magnetic tape. The signal collector consists of photomultiplier tubes implanted in a cassegrain telescope. Flight tests of the system involved on-measurements at 285.95 nm and off-measurements at 299.40 nm, which yielded a differential cross section of 1.74 x 10 to the -16th sq cm. In situ measurements with another plane at a nominal altitude of 3.2 km for comparison purposes showed accuracy to within 10% in and above the boundary layer. The system is considered as a test apparatus for more developed versions to be flown on the Shuttle
TL;DR: A 2 microm wavelength, 90 mJ, 5 Hz pulsed Ho laser is described with wavelength control to precisely tune and lock the wavelength at a desired offset up to 2.9 GHz from the center of a CO(2) absorption line.
Abstract: A 2 μm wavelength, 90 mJ, 5 Hz pulsed Ho laser is described with wavelength control to precisely tune and lock the wavelength at a desired offset up to 29 GHz from the center of a CO2 absorption line Once detuned from the line center the laser wavelength is actively locked to keep the wavelength within 19 MHz standard deviation about the setpoint This wavelength control allows optimization of the optical depth for a differential absorption lidar (DIAL) measuring atmospheric CO2 concentrations The laser transmitter has been coupled with a coherent heterodyne receiver for measurements of CO2 concentration using aerosol backscatter; wind and aerosols are also measured with the same lidar and provide useful additional information on atmospheric structure Range-resolved CO2 measurements were made with <24% standard deviation using 500 m range bins and 67 min (1000 pulse pairs) integration time Measurement of a horizontal column showed a precision of the CO2 concentration to <07% standard deviation using a 30 min (4500 pulse pairs) integration time, and comparison with a collocated in situ sensor showed the DIAL to measure the same trend of a diurnal variation and to detect shorter time scale CO2 perturbations For vertical column measurements the lidar was setup at the WLEF tall tower site in Wisconsin to provide meteorological profiles and to compare the DIAL measurements with the in situ sensors distributed on the tower up to 396 m height Assuming the DIAL column measurement extending from 153 m altitude to 1353 m altitude should agree with the tower in situ sensor at 396 m altitude, there was a 79 ppm rms difference between the DIAL and the in situ sensor using a 30 min rolling average on the DIAL measurement
TL;DR: Comparisons are made between the water vapor DIAL measurements and data obtained from locally launched rawinsondes, and agreement was found to be within the uncertainty of the rawinsonde data to an altitude of 3 km.
Abstract: A ground-based differential absorption lidar (DIAL) system is described which has been developed for vertical range-resolved measurements of water vapor. The laser transmitter consists of a ruby-pumped dye laser, which is operated on a water vapor absorption line at 724.372 nm. Part of the ruby laser output is transmitted simultaneously with the dye laser output to determine atmospheric scattering and attenuation characteristics. The dye and ruby laser backscattered light is collected by a 0.5-m diam telescope, optically separated in the receiver package, and independently detected using photomultiplier tubes. Measurements of vertical water vapor concentration profiles using the DIAL system at night are discussed, and comparisons are made between the water vapor DIAL measurements and data obtained from locally launched rawinsondes. Agreement between these measurements was found to be within the uncertainty of the rawinsonde data to an altitude of 3 km. Theoretical simulations of this measurement were found to give reasonably accurate predictions of the random error of the DIAL measurements. Confidence in these calculations will permit the design of aircraft and Shuttle DIAL systems and experiments using simulation results as the basis for defining lidar system performance requirements.