Tackling orientation of metal-organic frameworks (MOFs): The quest to enhance MOF performance
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TL;DR: In this paper , the authors summarized the strategies utilized for the preparation and growth of oriented anisotropic metal-organic frameworks (MOFs) and highlighted the possibilities of each synthetic approach as well as the challenges they have to overcome.
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About: This article is published in Coordination Chemistry Reviews. The article was published on 01 Apr 2023. and is currently open access. The article focuses on the topics: Metal-organic framework & Chemistry.
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Citations
Understanding and controlling the nucleation and growth of metal-organic frameworks.
Brooke P Carpenter,A. R. Talosig,Ben Rose,Giuseppe Di Palma,Joseph Patrick Patterson +4 more
TL;DR: This review synthesizes current theories and chemistry of metal-organic framework (MOF) crystallization, discussing intrinsic and extrinsic parameters to modulate crystallization pathways and produce MOFs with tailored properties through experimental and computational methods.
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Electrocatalytic Synthesis of Pyridine Oximes using in Situ Generated NH2OH from NO species on Nanofiber Membranes Derived from NH2-MIL-53(Al).
Runan Xiang,Shih Chuan Wang,Peisen Liao,Fangyan Xie,Jiawei Kang,Suisheng Li,Jiahui Xian,Lina Guo,Guangqin Li +8 more
- 20 Sep 2023
TL;DR: Electrocatalytic synthesis of pyridine oximes using in situ generated NH2OH from NO species on nanofiber membranes derived from NH2-MIL-53(Al) directly synthesizes pyridine oximes using in situ generated NH2OH from NO reduction with well-designed nanofiber membranes derived from NH2-MIL-53(Al).
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Fabrication of Oriented Polycrystalline MOF Superstructures.
Mercedes Linares-Moreau,Lea A. Brandner,Miriam de J. Velásquez-Hernández,Javier Fonseca,Youven Benseghir,Jia Min Chin,Daniel Maspoch,Christian J. Doonan,Paolo Falcaro +8 more
TL;DR: Fabrication of oriented polycrystalline MOF superstructures focuses on aligning the pore channels of MOF crystals in specific directions, leading to anisotropic properties.
32
Dual‐step Redox Engineering of Two‐Dimensional CoNi‐Alloy Embedded B, N‐Doped Carbon Layers towards Tunable Electromagnetic Wave Absorption and Light‐Weight Infrared Stealth Heat Insulation Devices
Wen‐Huan Huang,Ming Song,Shun Wang,Bokun Wang,Jiachen Ma,Tong Liu,Yanan Zhang,Yifan Kang,Renchao Che +8 more
TL;DR: Dual-step redox engineering of 2D-CoNi-alloy embedded B, N-doped carbon layers for tunable electromagnetic wave absorption and lightweight infrared stealth heat insulation devices.
31
Construction of the copper metal-organic framework (MOF)-on-indium MOF Z-scheme heterojunction for efficiently photocatalytic reduction of Cr(VI)
Jia-Yue Tian,Wenmiao Lv,Ao-Song Shen,Yashen Ma,Minghua Wang,Shuai Zhang,Xiao-Long Liu,Zhihong Zhang,Miao Du +8 more
TL;DR: A novel 2D-on-3D MOF heterostructure, Cu-MOF@In-MOF, was synthesized and demonstrated enhanced photocatalytic reduction efficiency (98%) of Cr(VI) under visible-light irradiation, outperforming sole MOFs and most reported photocatalysts.
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References
The Chemistry and Applications of Metal-Organic Frameworks
Hiroyasu Furukawa,Hiroyasu Furukawa,Kyle E. Cordova,Kyle E. Cordova,Michael O'Keeffe,Michael O'Keeffe,Omar M. Yaghi,Omar M. Yaghi,Omar M. Yaghi +8 more
TL;DR: Metal-organic frameworks are porous materials that have potential for applications such as gas storage and separation, as well as catalysis, and methods are being developed for making nanocrystals and supercrystals of MOFs for their incorporation into devices.
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Mussel-Inspired Surface Chemistry for Multifunctional Coatings
TL;DR: Inspired by the composition of adhesive proteins in mussels, dopamine self-polymerization is used to form thin, surface-adherent polydopamine films onto a wide range of inorganic and organic materials, including noble metals, oxides, polymers, semiconductors, and ceramics.
Formation and Structure of Self-Assembled Monolayers.
TL;DR: Monolayers of alkanethiolates on gold are probably the most studied SAMs to date and offer the needed design flexibility, both at the individual molecular and at the material levels, and offer a vehicle for investigation of specific interactions at interfaces, and of the effect of increasing molecular complexity on the structure and stability of two-dimensional assemblies.
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