Journal Article10.1021/acs.nanolett.3c00460
Electric-Field-Driven Trion Drift and Funneling in MoSe2 Monolayer.
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TL;DR: In this paper , the authors demonstrate electric-field-driven drift and funneling of charged excitons (i.e., trions) toward the center of a MoSe2 monolayer.
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Abstract: Excitons, electron-hole pairs in semiconductors, can be utilized as information carriers with a spin or valley degree of freedom. However, manipulation of excitons' motion is challenging because of their charge-neutral characteristic and short recombination lifetimes. Here we demonstrate electric-field-driven drift and funneling of charged excitons (i.e., trions) toward the center of a MoSe2 monolayer. Using a simple bottom-gate device, we control the electric fields in the vicinity of the suspended monolayer, which increases the trion density and pulls down the layer. We observe that locally excited trions are subjected to electric force and, consequently, drift toward the center of the stretched layer. The exerting electric force on the trion is estimated to be 102-104 times stronger than the strain-induced force in the stretched monolayer, leading to the successful observation of trion drift under continuous-wave excitation. Our findings provide a new route for manipulating trions and achieving new types of optoelectronic devices.
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Citations
Recent progress of exciton transport in two-dimensional semiconductors
Hyeongwoo Lee,Yong Bin Kim,Jae Won Ryu,Sujeong Kim,Jinhyuk Bae,Yeonjeong Koo,Donghoon Jang,Kyoung-Duck Park +7 more
TL;DR: This review summarizes recent advancements in controlling exciton currents in 2D semiconductors using electric fields, strain gradients, surface plasmon polaritons, and photonic cavities, addressing challenges in exciton transport for optoelectronic applications.
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Nanoscale Manipulation of Exciton-Trion Interconversion in a MoSe2 Monolayer via Tip-Enhanced Cavity-Spectroscopy.
Mingu Kang,Su Jin Kim,Huitae Joo,Yeonjeong Koo,Hyeongwoo Lee,Hyun Seok Lee,Yung Doug Suh,Kyoung-Duck Park +7 more
- 20 Dec 2023
TL;DR: Plasmon-induced near-field manipulation of exciton-trion interconversion in a MoSe2 monolayer using tip-enhanced cavity-spectroscopy enables nanoscale control of X0 and X- populations and dynamic interconversion between X0 and X- at the nanoscale.
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