Journal Article10.1002/CSSC.201000447
Chemical Technologies for Exploiting and Recycling Carbon Dioxide into the Value Chain
Martina Peters,Martina Peters,Burkhard Köhler,Wilhelm Kuckshinrichs,Walter Leitner,Peter Markewitz,Thomas Müller +6 more
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TL;DR: Carbon dioxide can be a promising carbon source with practically unlimited availability for a range of industrially relevant products and can be used as a versatile processing fluid based on its remarkable physicochemical properties.
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Abstract: While experts in various fields discuss the potential of carbon capture and storage (CCS) technologies, the utilization of carbon dioxide as chemical feedstock is also attracting renewed and rapidly growing interest. These approaches do not compete; rather, they are complementary: CCS aims to capture and store huge quantities of carbon dioxide, while the chemical exploitation of carbon dioxide aims to generate value and develop better and more-efficient processes from a limited part of the waste stream. Provided that the overall carbon footprint for the carbon dioxide-based process chain is competitive with conventional chemical production and that the reaction with the carbon dioxide molecule is enabled by the use of appropriate catalysts, carbon dioxide can be a promising carbon source with practically unlimited availability for a range of industrially relevant products. In addition, it can be used as a versatile processing fluid based on its remarkable physicochemical properties.
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Citations
Carbon capture and storage (CCS): the way forward
Mai Bui,Claire S. Adjiman,André Bardow,Edward J. Anthony,Andy Boston,Solomon Brown,Paul S. Fennell,Sabine Fuss,Amparo Galindo,Leigh A. Hackett,Jason P. Hallett,Howard J. Herzog,George Jackson,Jasmin Kemper,Samuel Krevor,Geoffrey C. Maitland,Michael Matuszewski,Ian S. Metcalfe,Camille Petit,Graeme Puxty,Jeffrey A. Reimer,David Reiner,Edward S. Rubin,Stuart A. Scott,Nilay Shah,Berend Smit,Berend Smit,J. P. Martin Trusler,Paul A. Webley,Jennifer Wilcox,Niall Mac Dowell +30 more
TL;DR: In this article, the authors review the current state-of-the-art of CO2 capture, transport, utilisation and storage from a multi-scale perspective, moving from the global to molecular scales.
Sustainable Conversion of Carbon Dioxide: An Integrated Review of Catalysis and Life Cycle Assessment
Jens Artz,Thomas Müller,Katharina Thenert,Johanna Kleinekorte,Raoul Meys,André Dirk Sternberg,André Bardow,Walter Leitner,Walter Leitner +8 more
TL;DR: The motivation to develop CO2-based chemistry does not depend primarily on the absolute amount of CO2 emissions that can be remediated by a single technology and is stimulated by the significance of the relative improvement in carbon balance and other critical factors defining the environmental impact of chemical production in all relevant sectors in accord with the principles of green chemistry.
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