Carbon Capture and Utilization Update
TL;DR: In this paper, the authors provide an overview of the current status of CO2-capture technologies and their associated challenges and opportunities with respect to efficiency and economy, and summarize the main challenges associated with the design, development, and large-scale deployment of new technologies and opportunities to accelerate their scaleup in the near future.
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Abstract: In recent years, carbon capture and utilization (CCU) has been proposed as a potential technological solution to the problems of greenhouse-gas emissions and the ever-growing energy demand. To combat climate change and ocean acidification as a result of anthropogenic CO2 emissions, efforts have already been put forth to capture and sequester CO2 from large point sources, especially power plants; however, the utilization of CO2 as a feedstock to make valuable chemicals, materials, and transportation fuels is potentially more desirable and provides a better and long-term solution than sequestration. The products of CO2 utilization can supplement or replace chemical feedstocks in the fine chemicals, pharmaceutical, and polymer industries. In this review, we first provide an overview of the current status of CO2-capture technologies and their associated challenges and opportunities with respect to efficiency and economy followed by an overview of various carbon-utilization approaches. The current status of combined CO2 capture and utilization, as a novel efficient and cost-effective approach, is also briefly discussed. We summarize the main challenges associated with the design, development, and large-scale deployment of CO2 capture and utilization processes to provide a perspective and roadmap for the development of new technologies and opportunities to accelerate their scale-up in the near future.
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Citations
Climate change mitigation potential of carbon capture and utilization in the chemical industry.
TL;DR: This study shows that CCU has the technical potential to lead to a carbon-neutral chemical industry and decouple chemical production from fossil resources, reducing annual GHG emissions by up to 3.5 Gt CO2-eq in 2030.
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Progress in carbon capture technologies.
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Semiconductor Quantum Dots: An Emerging Candidate for CO2 Photoreduction.
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The future of hydrogen: Challenges on production, storage and applications
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Advances and challenges in electrochemical CO2 reduction processes: an engineering and design perspective looking beyond new catalyst materials
Sahil Garg,Mengran Li,Adam Z. Weber,Lei Ge,Lei Ge,Liye Li,Victor Rudolph,Guoxiong Wang,Thomas E. Rufford +8 more
TL;DR: In this article, the authors examine the state-of-the-art in electrochemical CO2 reduction technologies, and highlight how the efficiency of CO2R processes can be improved through (i) electrolyzer configuration, (ii) electrode structure, (iii) electrolyte selection, pH control, and (iv) the electrolyzer's operating pressure and temperature.
References
Amine Scrubbing for CO2 Capture
TL;DR: Amine scrubbing has been used to separate carbon dioxide (CO2) from natural gas and hydrogen since 1930 and is ready to be tested and used on a larger scale for CO2 capture from coal-fired power plants.
3.9K
Adsorbent Materials for Carbon Dioxide Capture from Large Anthropogenic Point Sources
TL;DR: The CO(2) adsorption behavior of several different classes of solid carbon dioxide adsorbents, including zeolites, activated carbons, calcium oxides, hydrotalcites, organic-inorganic hybrids, and metal-organic frameworks are described.
2.4K
Synthesis, Structure, and Carbon Dioxide Capture Properties of Zeolitic Imidazolate Frameworks
Anh Phan,Christian J. Doonan,Fernando J. Uribe-Romo,Carolyn B. Knobler,Michael O'Keeffe,Omar M. Yaghi +5 more
TL;DR: The general preparation of crystalline ZIFs is described, discussing the methods that have been developed to create and analyze the variety of materials afforded and how complexity might be introduced into new structures.
CO2 Capture by a Task-Specific Ionic Liquid
TL;DR: A new room temperature ionic liquid incorporating a cation with an appended amine group is produced, comparable in efficiency for CO2 capture to commercial amine sequestering reagents, and yet is nonvolatile and does not require water to function.
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