Photonics and thermodynamics concepts in radiative cooling

Abstract To fight against global warming, subambient daytime radiative cooling technology provides a promising path to meet sustainable development goals. To achieve subambient daytime radiative cooling, the reflection of most sunlight is the essential prerequisite. However, the desired high solar reflectance is easily dampened by environmental aging, mainly natural soiling and ultraviolet irradiation from sunlight causing yellowish color for most polymers, making the cooling ineffective. We demonstrate a simple strategy to use titanium dioxide nanoparticles, with ultraviolet resistance, forming hierarchical porous morphology via evaporation-driven assembly, which guarantees a balanced anti-soiling and high solar reflectance, rendering anti-aging cooling paint based coatings. We challenge the cooling coatings in an accelerated weathering test against simulated 3 years of natural soiling and simulated 1 year of natural sunshine, and find that the solar reflectance only declined by 0.4% and 0.5% compared with the un-aged ones. We further show over 6 months of aging under real-world conditions with barely no degradation to the cooling performance. Our anti-aging cooling paint is scalable and can be spray coated on desired outdoor architecture and container, presenting durable radiative cooling, promising for real-world applications. 

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Durable radiative cooling against environmental aging

The seamless integration of emerging triboelectric nanogenerator (TENG) technology with traditional wearable textile materials has given birth to the next‐generation smart textiles, i.e., textile TENGs, which will play a vital role in the era of Internet of Things and artificial intelligences. However, low output power and inferior sensing ability have largely limited the development of textile TENGs. Among various approaches to improve the output and sensing performance, such as material modification, structural design, and environmental management, a 3D fabric structural scheme is a facile, efficient, controllable, and scalable strategy to increase the effective contact area for contact electrification of textile TENGs without cumbersome material processing and service area restrictions. Herein, the recent advances of the current reported textile TENGs with 3D fabric structures are comprehensively summarized and systematically analyzed in order to clarify their superiorities over 1D fiber and 2D fabric structures in terms of power output and pressure sensing. The forward‐looking integration abilities of the 3D fabrics are also discussed at the end. It is believed that the overview and analysis of textile TENGs with distinctive 3D fabric structures will contribute to the development and realization of high‐power output micro/nanowearable power sources and high‐quality self‐powered wearable sensors.

Advances in High‐Performance Autonomous Energy and Self‐Powered Sensing Textiles with Novel 3D Fabric Structures

Developing functional textiles with a cooling effect is important for personal comfort in human life and activities. Although existing passive cooling fabrics exhibit promising cooling effects, they do not meet the thermal comfort requirements under many practical conditions. Here, we report a nanofiber membrane-based moisture-wicking passive cooling hierarchical metafabric that couples selective optical cooling and wick-evaporation cooling to achieve efficient temperature and moisture management. The hierarchical metafabric showed high sunlight reflectivity (99.16% in the 0.3-0.76 μm wavelength range and 88.60% in the 0.76-2.5 μm wavelength range), selective infrared emissivity (78.13% in the 8-13 μm wavelength range), and good moisture permeability owing to the optical properties of the material and hierarchical morphology design. Cooling performance experiments revealed that covering simulated skin with the hierarchical metafabric prevented overheating by 16.6 °C compared with traditional textiles, including a contribution from management of the humidity (∼8.2 °C). In addition to the personal thermal management ability, the hierarchical metafabric also showed good wearability.

A Moisture-Wicking Passive Radiative Cooling Hierarchical Metafabric.

Personal cooling textiles are a promising energy-free pathway for confronting serious heat-related public health threats and improving industrial worker productivity. Current cooling strategies mainly focus on passive daytime radiation, and there is a lack of research on all-day cooling methods which utilize synergistic radiative, conductive, and evaporative heat dissipation. Herein, we demonstrate a hierarchical polyurethane/silicon nitride fibrous membrane with Janus wettability fabricated via a scalable electrospinning method followed by single-side hydrophilic plasma treatment. High angular-dependent solar reflectance (91%) and human body infrared emittance (93%) allow for a temperature drop of ∼21.9 °C under direct sunlight and ∼2.8 °C at night compared with traditional cotton. The innovative integration of Janus wettability and heat conduction in hierarchically designed textiles ensures a minimum sweat consumption of 0.5 mL h-1, avoiding harmfully excessive perspiration. The excellent all-day cooling performance of this hierarchical textile presents great advantages for smart textile, energy-saving, and personal cooling applications.

Integration of Janus Wettability and Heat Conduction in Hierarchically Designed Textiles for All-Day Personal Radiative Cooling.

Incorporating passive radiative cooling structures into personal thermal management technologies could effectively defend humans against intensifying global climate change. We show that large-scale woven metafabrics can provide high emissivity (94.5%) in the atmospheric window and high reflectivity (92.4%) in the solar spectrum because of the hierarchical-morphology design of the randomly dispersed scatterers throughout the metafabric. Through scalable industrial textile manufacturing routes, our metafabrics exhibit desirable mechanical strength, waterproofness, and breathability for commercial clothing while maintaining efficient radiative cooling ability. Practical application tests demonstrated that a human body covered by our metafabric could be cooled ~4.8°C lower than one covered by commercial cotton fabric. The cost-effectiveness and high performance of our metafabrics present substantial advantages for intelligent garments, smart textiles, and passive radiative cooling applications.

Hierarchical-morphology metafabric for scalable passive daytime radiative cooling.

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Hierarchical-morphology metafabric for scalable passive daytime radiative cooling.