Ordered mesoporous materials prepared by the template route have attracted increasing interest from the electrochemists community due to their plenty of unique properties and functionalities that can be effectively exploited in electrochemical devices. This review will cover the whole field of the intersection between electrochemistry and ordered mesoporous materials. The latter are either electronically insulating (silica and some other metal oxides, as well as silica-based organic–inorganic hybrid materials), semi-conducting (metal oxides), or conducting (metals, carbons). The three main intersection areas are: (1) the development/use of electrochemical methods to characterize the properties of mesoporous materials (i.e., charge and mass transfer processes); (2) the generation of mesostructured solids by electro-assisted deposition using appropriate templates; and (3) the application of these novel materials for electrochemical purposes. The most common devices to date are based on a bulk composite or thin film configuration and the resulting electrodes modified with such mesoporous materials have been successfully applied in various fields, including mainly electrochemical sensing and biosensing as well as energy conversion and storage (620 references).

Mesoporous materials and electrochemistry

A review on electrodes modified with ionic liquids

Prussian blue (PB), the oldest synthetic coordination compound, is a classic and fascinating transition metal coordination material. Prussian blue is based on a three-dimensional (3-D) cubic polymeric porous network consisting of alternating ferric and ferrous ions, which provides facile assembly as well as precise interaction with active sites at functional interfaces. A fundamental understanding of the assembly mechanism of PB hetero-interfaces is essential to enable the full potential applications of PB crystals, including chemical sensing, catalysis, gas storage, drug delivery and electronic displays. Developing controlled assembly methods towards functionally integrated hetero-interfaces with adjustable sizes and morphology of PB crystals is necessary. A key point in the functional interface and device integration of PB nanocrystals is the fabrication of hetero-interfaces in a well-defined and oriented fashion on given substrates. This review will bring together these key aspects of the hetero-interfaces of PB nanocrystals, ranging from structure and properties, interfacial assembly strategies, to integrated hetero-structures for diverse sensing.

New faces of porous Prussian blue: interfacial assembly of integrated hetero-structures for sensing applications.

Conducting polymer-noble metal nanoparticle hybrids: Synthesis mechanism application

https://orbit.dtu.dk/files/5788619/elsevier%5B1%5D.pdf

Layer-by-layer assembled multilayer of graphene/Prussian blue toward simultaneous electrochemical and SPR detection of H2O2

Fabrication and electrochemical characterization of electrostatic assembly of polyelectrolyte-functionalized ionic liquid and Prussian blue ultrathin films

Controlled synthesis of nanoporous Au microsheet via surfactant emulsion template

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Fabrication and electrochemical characterization of electrostatic assembly of polyelectrolyte-functionalized ionic liquid and Prussian blue ultrathin films

Controlled synthesis of nanoporous Au microsheet via surfactant emulsion template