The stratospheric contribution to tropospheric ozone has long been a topic of much debate over the past few decades. In this study, we leveraged multiple datasets from surface, sounding and satellite observations to reanalysis datasets, along with a global chemical transport model (Global Nested Air Quality Prediction Modelling System, GNAQPMS) to investigate the impact of a stratospheric-to-tropospheric transport (STT) event characterized by long duration and wide range in the summer on surface high ozone episodes over heavily industrialized regions in northern China. In 14–18 August 2019, the ERA5 reanalysis datasets showed a potential vorticity (PV) tongue and a deep, upper-level trough penetrate towards 35° N over the North China Plain (NCP), indicating the occurrence of a stratospheric intrusion. From Atmospheric Infrared Sounder (AIRS) measurements, we found that the ozone-rich, stratospheric air mass had been injected into the lower altitudes. The GNAQPMS generally captured the featured layers, although there was a slight underestimation in the low troposphere. The averaged magnitudes of stratospheric contribution (O3S) and percentage (O3F) simulated by GNAQPMS were 3–20 μg m−3 and 6%–20%, respectively, while the Whole Atmosphere Community Climate Model (WACCM) indicated a higher stratospheric contribution by 3–5 μg m−3. Through this study, we give our opinions on the controversial topic of a more thorough understanding of the influence of natural processes apart from anthropogenic emissions, even in a heavily polluted region during summer.

Influences of stratospheric intrusions to high summer surface ozone over a heavily industrialized region in northern China

With climate warming, eastern China has experienced a significant increase in temperature accompanied by intensified ozone pollution. We aimed to investigate the spatiotemporal patterns and relationships between ozone levels and temperature in eastern China using observation-based ozone data from 418 air quality monitoring stations and temperature data from ERA5. The summer maximum temperature and annual ozone concentration in eastern China increased significantly between 2015 and 2022, with increases rate of 10% and 2.84 μg/m3 yr-1, respectively. The baseline ozone concentration was increasing over time. The average difference in MDA8 O3 concentration in spring, summer, and autumn decreased, with more ozone pollution spreading into spring and autumn, indicating a trend of prolonging the ozone season. During the June-July-August (JJA) period of 2015-2022, heatwaves increased significantly in eastern China. The frequency of heatwave events >10 days played a vital role in exacerbating ozone pollution. During the JJA period, the increase rate in MDA8 O3 concentration was 9.31 μg/m3 yr-1 during heatwave periods, significantly higher than that during non-heatwave periods (4.01 μg/m3 yr-1). The correlation between MDA8 O3 concentration and temperature was as high as 0.99, indicating that temperature was vital in ozone formation during the JJA period in eastern China. This study suggests that more stringent actions are needed to control ozone-precursor compounds during frequent summertime heatwaves in eastern China. 

Evolution of surface ozone pollution pattern in eastern China and its relationship with different intensity heatwaves.

In recent years, ozone (O3) concentration has shown a decreasing trend in the Beijing–Tianjin–Hebei (BTH) region in China. However, O3 pollution remains a prominent problem. Accurate estimation of O3 exposure levels can provide support for epidemiological studies. A total of 13 variables were combined to estimate short- and long-term O3 exposure levels using the geographically weighted regression (GWR) model in the BTH region with a spatial resolution of 1 × 1 km from 2017 to 2020. Five variables were left in the GWR model. O3 concentration was positively correlated with temperature, wind speed, and SO2, whereas is was negatively correlated with precipitation and NO2. Results showed that the model performed well. Leave-one-out cross-validation (LOOCV) R2 for short- and long-term simulation results were 0.91 and 0.71, and the values for RMSE were 11.14 and 3.49 μg/m3, respectively. The annual maximum 8 h average O3 concentration was the highest in 2018 and the lowest in 2020. Decreasing concentrations of major precursors of O3 due to the regional joint prevention and control may be the reason. O3 concentration was high in the southeast of the BTH region, including in Hengshui, Handan, Xingtai and Cangzhou.

/pdf/estimation-of-short-term-and-long-term-ozone-exposure-levels-18uo5q4o.pdf

Estimation of Short-Term and Long-Term Ozone Exposure Levels in Beijing–Tianjin–Hebei Region Based on Geographically Weighted Regression Model

Remote Sensing of Tropospheric Ozone From Space: Progress and Challenges

Liver-specific actions of GH and IGF1 that protect against MASLD.

Satellite monitoring of stratospheric ozone intrusion exceptional events- a typical case of China in 2019

http://www.ygxb.ac.cn/rc-pub/front/front-article/download?siteId=91&id=24627741&attachType=lowqualitypdf&token=&language=zh

Advances of ozone satellite remote sensing in 60 years

ABSTRACT Both growth hormone (GH) and gut microbiota play significant roles in diverse physiological processes, but the crosstalk between them is poorly understood. Despite the regulation of GH by gut microbiota, study on GH’s influence on gut microbiota is limited, especially on the impacts of tissue specific GH signaling and their feedback effects on the host. In this study, we profiled gut microbiota and metabolome in tissue-specific GHR knockout mice in the liver (LKO) and adipose tissue (AKO). We found that GHR disruption in the liver rather than adipose tissue affected gut microbiota. It changed the abundance of Bacteroidota and Firmicutes at phylum level as well as abundance of several genera, such as Lactobacillus, Muribaculaceae, and Parasutterella, without affecting α-diversity. Moreover, the impaired liver bile acid (BA) profile in LKO mice was strongly associated with the change of gut microbiota. The BA pools and 12-OH BAs/non-12-OH BAs ratio were increased in the LKO mice, which was due to the induction of CYP8B1 by hepatic Ghr knockout. Consequently, the impaired BA pool in cecal content interacted with gut bacteria, which in turn increased the production of bacteria derived acetic acid, propionic acid, and phenylacetic acid that were possible to participate in the impaired metabolic phenotype of the LKO mice. Collectively, our findings suggested that the liver GH signaling regulates BA metabolism by its direct regulation on CYP8B1, which is an important factor influencing gut microbiota. Our study is significant in exploring gut microbiota modification effects of tissue-specific GH signaling as well as its involvement in gut microbiota–host interaction.

https://www.tandfonline.com/doi/pdf/10.1080/19490976.2023.2221098?needAccess=true&role=button

Deletion of hepatic growth hormone receptor (GHR) alters the mouse gut microbiota by affecting bile acid metabolism

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Satellite monitoring of stratospheric ozone intrusion exceptional events- a typical case of China in 2019

Advances of ozone satellite remote sensing in 60 years

Deletion of hepatic growth hormone receptor (GHR) alters the mouse gut microbiota by affecting bile acid metabolism