We report the magnetic changes from canted antiferromagnetic to ferromagnetic orderings in anti-115-type MnPt 5- x Pd x P ( x = 1, 2, 2.5, 3, 4, and 5) and the discovery of a new rare-earth-free ferromagnet, MnPd 5 P by both theoretical prediction and experimental investigation. The family compounds were synthesized using high temperature solid state method and characterized to crystalize in the anti-CeCoIn 5 type with the space group P 4/ mmm exhibiting a two-dimensional layered structural feature. The magnetic property measurements indicate that the compounds ordered from canted A-type antiferromagnet in MnPt 5 P to ferromagnet above the room temperature with varying degrees of coercivity and magnetic moments in MnPd 5 P by reducing the spin orbital coupling. The results of the MnPt 5- x Pd x P have been analyzed in comparison to the other candidates of the 151 family of Mn(Pt/Pd) 5 (P/As) to understand the complex structure-magnetism relationships.

Theory-guided investigation on magnetic evolution of MnPt$_{5-x}$Pd$_x$P and discovery of anti-CeCoIn$_5$-type ferromagnetic MnPd$_5$P

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Theory-guided investigation on magnetic evolution of MnPt$_{5-x}$Pd$_x$P and discovery of anti-CeCoIn$_5$-type ferromagnetic MnPd$_5$P