Strongly luminescent and highly stable CsPbBr3/Cs4PbBr6 core/shell nanocrystals and their ultrafast carrier dynamics

Inorganic lead halide perovskite is one of the most excellent fluorescent materials, and it plays an essential role in high-definition display and visible light communication (VLC). Its photochromic properties and stability determine the final performance of light-emitting devices. However, efficiently synthesizing perovskite with high quality and stability remains a significant challenge. Here, we develop a facile and environmentally friendly method for preparing high-stability and strong-emission CsPbBr3/Cs4PbBr6 composites using ultrasonication and liquid paraffin. Tuning the contents of liquid paraffin, bright-emission CsPbBr3/Cs4PbBr6 composite powders with a maximum PLQY of 74% were achieved. Thanks to the protection of the Cs4PbBr6 matrix and liquid paraffin, the photostability, thermostability, and polar solvent stability of CsPbBr3/Cs4PbBr6-LP are significantly improved compared to CsPbBr3 quantum dots and CsPbBr3/Cs4PbBr6 composites that were prepared without liquid paraffin. Moreover, the fabricated CsPbBr3/Cs4PbBr6-LP-based WLEDs show excellent luminescent performance with a power efficiency of 129.5 lm/W and a wide color gamut, with 121% of the NTSC and 94% of the Rec. 2020, demonstrating a promising candidate for displays. In addition, the CsPbBr3/Cs4PbBr6-LP-based WLEDs were also demonstrated in a VLC system. The results suggested the great potential of these high-performance WLEDs as an excitation light source to achieve VLC.

/pdf/highly-stable-and-photoluminescent-cspbbr3-cs4pbbr6-2ym0fyz5.pdf

Highly Stable and Photoluminescent CsPbBr3/Cs4PbBr6 Composites for White-Light-Emitting Diodes and Visible Light Communication

Organic polystyrene and inorganic silica double shell protected lead halide perovskite nanocrystals with high emission efficiency and superior stability

Carbon dots (CDs) are attracting much interest due to their excellent photoelectric properties and wide range of potential applications. However, it is still a challenge to regulate their bandgap emissions to achieve full-color CDs with high emissions. Herein, we propose an approach for producing full-color emissive CDs by employing a solvent engineering strategy. By only tuning the volume ratio of water and dimethylformamide (H2O/DMF), the photoluminescence (PL) emission wavelengths of the CDs can be changed from 451 to 654 nm. Different fluorescence features of multicolor CDs were systematically investigated. XRD, SEM, TEM, Abs/PL/PLE, XPS, and PL decay lifetime characterizations provided conclusive evidence supporting the extent to which the solvent controlled the dehydration and carbonization processes of the precursors, leading to a variation in their emission color from red to blue. The as-prepared CDs exhibited excellent and stable fluorescence performance even after being heated at 80 °C for 48 h and with UV light continuously irradiated for 15 h. Based on their excellent fluorescent properties and photothermal stability, bright multicolor light-emitting diodes with a high CRI of up to 91 were obtained. We anticipate that these full-color emissive CDs are beneficial for applications in lighting, display, and other fields.

/pdf/multicolor-luminescent-carbon-dots-tunable-photoluminescence-twjvrhfm.pdf

Multicolor Luminescent Carbon Dots: Tunable Photoluminescence, Excellent Stability, and Their Application in Light-Emitting Diodes

All-inorganic metal halide perovskites have been actively investigated as promising energy-converting materials for abundant applications owing to their excellent electronic and optical properties. Three-dimensional (3D) CsPbBr3, two-dimensional (2D) CsPb2Br5, and...

Phase engineering of inorganic halide Cs-Pb-Br perovskites for advanced energy conversion

CsPbBr3/Cs4PbBr6 heterostructure solids with high stability and photoluminescence for white light-emitting diodes

Precise regulation of the multicolor spectrum of carbon dots based on the bionic leaf vein ultrasonic microreactor

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CsPbBr3/Cs4PbBr6 heterostructure solids with high stability and photoluminescence for white light-emitting diodes

Precise regulation of the multicolor spectrum of carbon dots based on the bionic leaf vein ultrasonic microreactor