Lithium extraction from liquid resources has drawn significanct attention owing to its abundant deposits. However, developing highly efficient Li+ adsorbent materials is still limited by the unclear chemical mechanism between...

Unraveling the Li+ desorption behavior and mechanism of Li4Ti5O12 with different facets to enhance lithium extraction

Implementation of novel pulsed laser ablation strategy to control the morphological growth and enrich the electrochemically active sites of multifunctional Ni–CuO electrocatalyst

Safe extended-range cycling of Li4Ti5O12-based anodes for ultra-high capacity thin film batteries

Unveiling the Formation Mechanism and Phase Purity Control of Nanostructured Li4Ti5O12 via a Hydrothermal Process

Chloroaluminate-ions driven all-organic rechargeable batteries

Nanostructured lithium titanate (LTO, Li4Ti5O12) has garnered immense attention as a prospective anode material that can sustain high charge–discharge rates, offer prolonged cycle life, and particu...

Nanostructured Li4Ti5O12 Anodes: Delineating the Impact of Morphology, Exposed Facets, and Phase Purity on the Performance§

Rechargeable Li-ion batteries although efficiently power small portable devices, implementation in electric vehicle mobility to assuage environmental concerns demand batteries possessing higher power densities and capacities while being compact and safer. Recent research is hence focused towards developing battery components that can sustain high charge-discharge rates while comprehensively addressing the safety issues. In our present research effort, attempts are made to investigate the role of different binders on the performance of nanostructured lithium titanate (LTO, Li4Ti5O12) anodes in half-cell configuration against Li-metal. Commercial nano-LTO, Super-P and polyvinylidene fluoride (PVdF) are used as reference materials for comparative appraisal. An endeavor is made to showcase the feasibility of water soluble binders: sodium alginate (Na-alginate) and sodium carboxymethyl cellulose (Na-CMC) for greener processing of the electrodes and evaluate the effect on specific capacity, reversibility, charge retention and adaptability towards faster charging rate in the half-cells assembled. Binders provide sufficient adhesion interconnecting the active particles as well as maintain proper contact with the current collector, thus imparting electrode integrity over multiple charge-discharge cycles. This apart, binders are understood to influence the conductivity of electrodes, electrolyte wetting behavior, formation of solid-electrolyte interface (SEI) and the charge-transfer across interfaces. A lower interfacial resistance can promote higher specific capacity, increase energy density, improve reversibility, etc. while restricting capacity fade even at high C-rates; and the role of binders is found to contribute significantly. Comprehensive analysis of electrochemical impedance data collected at the end of each galvanostatic charge/discharge cycle provided crucial clues in understanding the charge transfer behavior for the electrodes fabricated with the binders.

Investigating alternate binders: Impact on the performance of lithium titanate anode

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Nanostructured Li4Ti5O12 Anodes: Delineating the Impact of Morphology, Exposed Facets, and Phase Purity on the Performance§

Investigating alternate binders: Impact on the performance of lithium titanate anode