In this work, we established a novel theory for the dynamics of oscillating bubbles such as cavitation bubbles, underwater explosion bubbles, and air bubbles. For the first time, we proposed bubble dynamics equations that can simultaneously take into consideration the effects of boundaries, bubble interaction, ambient flow field, gravity, bubble migration, fluid compressibility, viscosity, and surface tension while maintaining a unified and elegant mathematical form. The present theory unifies different classical bubble equations such as the Rayleigh-Plesset equation, the Gilmore equation, and the Keller-Miksis equation. Furthermore, we validated the theory with experimental data of bubbles with a variety in scales, sources, boundaries, and ambient conditions and showed the advantages of our theory over the classical theoretical models, followed by a discussion on the applicability of the present theory based on a comparison to simulation results with different numerical methods. Finally, as a demonstration of the potential of our theory, we modeled the complex multi-cycle bubble interaction with wide ranges of energy and phase differences and gained new physical insights into inter-bubble energy transfer and coupling of bubble-induced pressure waves.

pdf/a-unified-theory-for-bubble-dynamics-1rgsc6f4.pdf

A unified theory for bubble dynamics

The dynamics of spherical laser-induced cavitation bubbles in water is investigated by plasma photography, time-resolved shadowgraphs, and single-shot probe beam scattering enabling to portray the transition from initial nonlinear to late linear oscillations. The frequency of late oscillations yields the bubble's gas content. Simulations with the Gilmore model using plasma size as input and oscillation times as fit parameter provide insights into experimentally not accessible bubble parameters and shock wave emission. The model is extended by a term covering the initial shock-driven acceleration of the bubble wall, an automated method determining shock front position and pressure decay, and an energy balance for the partitioning of absorbed laser energy into vaporization, bubble and shock wave energy, and dissipation through viscosity and condensation. These tools are used for analysing a scattering signal covering 102 oscillation cycles. The bubble was produced by a plasma with 1550 K average temperature and had 36 $\mu$m maximum radius. Predicted bubble wall velocities during expansion agree well with experimental data. Upon first collapse, most energy was stored in the compressed liquid around the bubble and then radiated away acoustically. The collapsed bubble contained more vapour than gas, and its pressure was 13.5 GPa. The pressure of the rebound shock wave initially decayed $\propto r^{-1.8}$, and energy dissipation at the shock front heated liquid near the bubble wall above the superheat limit. The shock-induced temperature rise reduces damping during late bubble oscillations. Bubble dynamics changes significantly for small bubbles with less than 10 $\mu$m radius. 

/pdf/comprehensive-analysis-of-spherical-bubble-oscillations-and-1wtubkb3.pdf

Comprehensive analysis of spherical bubble oscillations and shock wave emission in laser-induced cavitation

The European XFEL delivers up to 27000 intense (>1012 photons) pulses per second, of ultrashort (≤50 fs) and transversely coherent X-ray radiation, at a maximum repetition rate of 4.5 MHz. Its unique X-ray beam parameters enable groundbreaking experiments in matter at extreme conditions at the High Energy Density (HED) scientific instrument. The performance of the HED instrument during its first two years of operation, its scientific remit, as well as ongoing installations towards full operation are presented. Scientific goals of HED include the investigation of extreme states of matter created by intense laser pulses, diamond anvil cells, or pulsed magnets, and ultrafast X-ray methods that allow their diagnosis using self-amplified spontaneous emission between 5 and 25 keV, coupled with X-ray monochromators and optional seeded beam operation. The HED instrument provides two target chambers, X-ray spectrometers for emission and scattering, X-ray detectors, and a timing tool to correct for residual timing jitter between laser and X-ray pulses.

/pdf/the-high-energy-density-scientific-instrument-at-the-2n432yhg7z.pdf

The High Energy Density Scientific Instrument at the European XFEL.

The Materials Imaging and Dynamics (MID) instrument at the European X-ray Free-Electron Laser (EuXFEL) facility is described. EuXFEL is the first hard X-ray free-electron laser operating in the MHz repetition range which provides novel science opportunities. The aim of MID is to enable studies of nano-structured materials, liquids, and soft- and hard-condensed matter using the bright X-ray beams generated by EuXFEL. Particular emphasis is on studies of structure and dynamics in materials by coherent scattering and imaging using hard X-rays. Commission of MID started at the end of 2018 and first experiments were performed in 2019.

/pdf/materials-imaging-and-dynamics-mid-instrument-at-the-1x45p3zthh.pdf

Materials Imaging and Dynamics (MID) instrument at the European X-ray Free-Electron Laser Facility.

Abstract This paper aims to use the unified bubble dynamics equation to investigate bubble behavior in complex scenarios involving hybrid free surface/wall boundaries and interactions between multiple bubbles. The effect of singularity movement on the unified equation’s form is analyzed after deriving the bubble pulsation equation using a moving point source and a dipole, followed by discussions on the effect of migration compressibility-related terms on the bubble dynamics. In addition, the present study accounts for the impact of hybrid boundaries, including crossed and parallel boundaries, by introducing a finite number of mirror bubbles for the former and an infinite number of mirror bubbles for the latter. Spark bubble experiments and numerical simulation are conducted to validate the present theory. The application of the unified equation in multi-bubble interactions is exemplified by computing a spherical bubble array containing more than 100 uniformly distributed cavitation bubbles under different boundary conditions. The bubble cluster-induced pressure peak can reach nearly two times or even higher than that of an individual bubble, highlighting the damage potential caused by cavitation bubble clusters. 

pdf/theoretical-study-on-bubble-dynamics-under-hybrid-boundary-4pcg9ja26u.pdf

Theoretical study on bubble dynamics under hybrid-boundary and multi-bubble conditions using the unified equation

X-ray free-electron lasers (XFELs) have opened up unprecedented opportunities for time-resolved nano-scale imaging with X-rays. Near-field propagation-based imaging, and in particular near-field holography (NFH) in its high-resolution implementation in cone-beam geometry, can offer full-field views of a specimen's dynamics captured by single XFEL pulses. To exploit this capability, for example in optical-pump/X-ray-probe imaging schemes, the stochastic nature of the self-amplified spontaneous emission pulses, i.e. the dynamics of the beam itself, presents a major challenge. In this work, a concept is presented to address the fluctuating illumination wavefronts by sampling the configuration space of SASE pulses before an actual recording, followed by a principal component analysis. This scheme is implemented at the MID (Materials Imaging and Dynamics) instrument of the European XFEL and time-resolved NFH is performed using aberration-corrected nano-focusing compound refractive lenses. Specifically, the dynamics of a micro-fluidic water-jet, which is commonly used as sample delivery system at XFELs, is imaged. The jet exhibits rich dynamics of droplet formation in the break-up regime. Moreover, pump–probe imaging is demonstrated using an infrared pulsed laser to induce cavitation and explosion of the jet.

/pdf/single-pulse-phase-contrast-imaging-at-free-electron-lasers-2xyjw1pisa.pdf

Single-pulse phase-contrast imaging at free-electron lasers in the hard X-ray regime

Single-pulse holographic imaging at XFEL sources with 1012 photons delivered in pulses shorter than 100 fs reveal new quantitative insights into fast phenomena. Here, a timing and synchronization scheme for stroboscopic imaging and quantitative analysis of fast phenomena on time scales (sub-ns) and length-scales (≲100 nm) inaccessible by visible light is reported. A fully electronic delay-and-trigger system has been implemented at the MID station at the European XFEL, and applied to the study of emerging laser-driven cavitation bubbles in water. Synchronization and timing precision have been characterized to be better than 1 ns.

/pdf/nanosecond-timing-and-synchronization-scheme-for-holographic-1kkwgwpfdn.pdf

Nanosecond timing and synchronization scheme for holographic pump-probe studies at the MID instrument at European XFEL.

Cavitation bubbles can be seeded from a plasma following optical breakdown, by focusing an intense laser in water. The fast dynamics are associated with extreme states of gas and liquid, especially in the nascent state. This offers a unique setting to probe water and water vapor far-from equilibrium. However, current optical techniques cannot quantify these early states due to contrast and resolution limitations. X-ray holography with single X-ray free-electron laser pulses has now enabled a quasi-instantaneous high resolution structural probe with contrast proportional to the electron density of the object. In this work, we demonstrate cone-beam holographic flash imaging of laser-induced cavitation bubbles in water with nanofocused X-ray free-electron laser pulses. We quantify the spatial and temporal pressure distribution of the shockwave surrounding the expanding cavitation bubble at time delays shortly after seeding and compare the results to numerical simulations.

/pdf/pump-probe-x-ray-holographic-imaging-of-laser-induced-3uxnf7r9gk.pdf

Pump-probe X-ray holographic imaging of laser-induced cavitation bubbles with femtosecond FEL pulses.

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Single-pulse phase-contrast imaging at free-electron lasers in the hard X-ray regime

Nanosecond timing and synchronization scheme for holographic pump-probe studies at the MID instrument at European XFEL.

Pump-probe X-ray holographic imaging of laser-induced cavitation bubbles with femtosecond FEL pulses.