Microengineering Pressure Sensor Active Layers for Improved Performance

CRISPR-Cas12a-driven MXene-PEDOT:PSS piezoresistive wireless biosensor

Photocatalytic water splitting, CO2 reduction, and pollutant degradation have emerged as promising strategies to remedy the existing environmental and energy crises. However, grafting of expensive and less abundant noble-metal cocatalysts on photocatalyst materials is a mandatory practice to achieve enhanced photocatalytic performance owing to the ability of the cocatalysts to extract electrons efficiently from the photocatalyst and enable rapid/enhanced catalytic reaction. Hence, developing highly efficient, inexpensive, and noble-metal-free cocatalysts composed of earth-abundant elements is considered as a noteworthy step toward considering photocatalysis as a more economical strategy. Recently, MXenes (two-dimensional (2D) transition-metal carbides, nitrides, and carbonitrides) have shown huge potential as alternatives for noble-metal cocatalysts. MXenes have several excellent properties, including atomically thin 2D morphology, metallic electrical conductivity, hydrophilic surface, and high specific surface area. In addition, they exhibit Gibbs free energy of intermediate H atom adsorption as close to zero and less than that of a commercial Pt-based cocatalyst, a Fermi level position above the H2 generation potential, and an excellent ability to capture and activate CO2 molecules. Therefore, there is a growing interest in MXene-based photocatalyst materials for various photocatalytic events. In this review, we focus on the recent advances in the synthesis of MXenes with 2D and 0D morphologies, the stability of MXenes, and MXene-based photocatalysts for H2 evolution, CO2 reduction, and pollutant degradation. The existing challenges and the possible future directions to enhance the photocatalytic performance of MXene-based photocatalysts are also discussed.

A Review on MXene Synthesis, Stability, and Photocatalytic Applications.

A self-powered temperature sensor based on Seebeck effect transduction was designed for photothermal–thermoelectric coupled immunoassay of α-fetoprotein (AFP). In this system, glucose oxidase (GOx)...

Self-Powered Temperature Sensor with Seebeck Effect Transduction for Photothermal–Thermoelectric Coupled Immunoassay

Flexible wearable sweat sensors allow continuous, real-time, noninvasive detection of sweat analytes, provide insight into human physiology at the molecular level, and have received significant attention for their promising applications in personalized health monitoring. Electrochemical sensors are the best choice for wearable sweat sensors due to their high performance, low cost, miniaturization, and wide applicability. Recent developments in soft microfluidics, multiplexed biosensing, energy harvesting devices, and materials have advanced the compatibility of wearable electrochemical sweat-sensing platforms. In this review, we summarize the potential of sweat for medical detection and methods for sweat stimulation and collection. This paper provides an overview of the components of wearable sweat sensors and recent developments in materials and power supply technologies and highlights some typical sensing platforms for different types of analytes. Finally, the paper ends with a discussion of the challenges and a view of the prospective development of this exciting field. 

/pdf/wearable-and-flexible-electrochemical-sensors-for-sweat-1w820kbe.pdf

Wearable and flexible electrochemical sensors for sweat analysis: a review

Methods based on the photothermal effect (a common phenomenon in nature) have been widely applied in different fields; however, their application in bioanalysis has lagged behind. Herein, we designed a near-infrared (NIR) photothermal immunoassay for the qualitative or quantitative detection of prostate-specific antigen (PSA) using titanium carbide (Ti3C2) MXene quantum dot (QD)-encapsulated liposomes with high photothermal efficiency. This system involves a sandwich-type immunoreaction and photothermal measurements. Ti3C2 MXene QDs were utilized as innovative photothermal signal beacons and were encapsulated in liposomes for the labeling of the secondary antibody. The assay was carried out by coupling a low-cost microplate with a homemade 3D printed device. Under NIR-laser irradiation, the Ti3C2 MXene QDs converted the light energy into heat, and a shift in temperature corresponding with the analyte concentration was obtained on a handheld thermometer. Under optimal conditions, the Ti3C2 MXene QD-based photothermal immunoassay exhibited a dynamic linear range from 1.0 ng mL-1 to 50 ng mL-1 with a limit of detection of 0.4 ng mL-1 for PSA detection. Also, we constructed portable equipment using a portable near-infrared imaging camera to collect visual thermal data for the semi-quantitative analysis of the target PSA within 3 min. The specificity, reproducibility and accuracy of the photothermal immunoassay were acceptable. Importantly, our strategy opens new opportunities for protein point-of-care (POC) testing and biosecurity diagnostics.

Ti3C2 MXene quantum dot-encapsulated liposomes for photothermal immunoassays using a portable near-infrared imaging camera on a smartphone.

A saw-toothed microstructure-based flexible pressure sensor was designed as the signal readout for point-of-care (POC) immunoassay of carcinoembryonic antigen (CEA). In this portable POC bioassay, the sandwich-type immunoreaction was first carried out to capture the target on a microplate, which simultaneously introduced the platinum nanoparticles (PtNPs). Upon adding hydrogen peroxide (H2O2), the pressure as the bridge between the molecular recognition event and detectable signal was increasing rapidly, resulting from the decomposition of H2O2 accelerated by PtNPs. Meanwhile, a flexible pressure sensor was fabricated with high sensitivity; the ability of the pressure response was dramatically improved by adopting the saw-toothed microstructure. By coupling with the pressure sensor, the pressure change could be monitored in real time to achieve the portable detection of CEA. Under the optimum conditions, the proposed pressure-based bioassay presented good sensing performance within 0.1-40 ng/mL at a detection limit of 87 pg/mL. The reproducibility, precision, and accuracy provided by the method were also studied and satisfied.

Saw-Toothed Microstructure-Based Flexible Pressure Sensor as the Signal Readout for Point-of-Care Immunoassay.

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Ti3C2 MXene quantum dot-encapsulated liposomes for photothermal immunoassays using a portable near-infrared imaging camera on a smartphone.

Saw-Toothed Microstructure-Based Flexible Pressure Sensor as the Signal Readout for Point-of-Care Immunoassay.