Metal hydrides are a class of materials that can absorb and release large amounts of hydrogen. They have a wide range of potential applications, including their use as a hydrogen storage medium for fuel cells or as a hydrogen release agent for chemical processing. While being a technology that can supersede existing energy storage systems in manifold ways, the use of metal hydrides also faces some challenges that currently hinder their widespread applicability. As the effectiveness of heat transfer across metal hydride systems can have a major impact on their overall efficiency, an affluent description of more efficient heat transfer systems is needed. The literature on the subject has proposed various methods that have been used to improve heat transfer in metal hydride systems over the years, such as optimization of the shape of the reactor vessel, the use of heat exchangers, phase change materials (PCM), nano oxide additives, adding cooling tubes and water jackets, and adding high thermal conductivity additives. This review article provides a comprehensive overview of the latest, state-of-the-art techniques in metal hydride reactor design and heat transfer enhancement methodologies and identifies key areas for future researchers to target. A comprehensive analysis of thermal management techniques is documented, including performance comparisons among various approaches and guidance on selecting appropriate thermal management techniques. For the comparisons, the hydrogen adsorption time relative to the reactor size and to the amount of hydrogen absorbed is studied. This review wishes to examine the various methods that have been used to improve heat transfer in metal hydride systems and thus aims to provide researchers and engineers working in the field of hydrogen storage with valuable insights and a roadmap to guide them to further explore the development of effective thermal management techniques for metal hydrides.

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Thermal Management Techniques in Metal Hydrides for Hydrogen Storage Applications: A Review

Design, development and hydrogen storage performance testing of a tube bundle metal hydride reactor

Hydrogen charging and discharging studies on embedded cooling tube metal hydride reactor designed for fuel cell applications

Metal hydride (MH) hydrogen storage systems have gained interest in the last decades. This review evaluates and compares the impact of thermal management measures on heat and mass transfer, summarizing the benefits and drawbacks of different reactor structures.

Review of thermal management technology for metal hydride reaction beds

Experimental studies on poisoning of La0.9Ce0.1Ni5 based hydrogen purification system with CO2 as impurity

• Heating and cooling traits of two AB 5 -type metal hydride alloys were investigated. • Heating performances of the alloys were found to be superior compared to cooling. • Peak heating rate of 3.5 kW was accomplished, producing 514 kJ heat within 361 s. • A decentralized heating cum H 2 storage system was suggested based on test results. The present work reports the heating and cooling characteristics of two AB 5 type metal hydride (MH) alloys commercially labelled as A3® and LCC1®. A cylindrical MH reactor configuration comprising 48 Embedded Cooling Tubes (ECT) in a circular pattern and an outer jacket was considered to accomplish the set objectives. Two identical reactors were each filled with 3.4 kg of one of the alloys. The reactor configuration allows MH alloy to be filled in the shell space while the heat transfer fluid (HTF) could flow through the tubes and the outer jacket. A set of parametric investigations was conducted on the aforementioned alloys by varying the operational parameters. During the absorption set of the parametric study, hydrogen supply pressure was varied from 10 bar to 30 bar, and HTF temperature was varied from 15 °C to 35 °C, while during the desorption study, HTF temperature was varied from 5 °C to 25 °C. At the absorption condition of 30 bar and 25 °C, the alloys A3® and LCC1® attained absorption capacity of 1.24 wt.% and 1.38 wt.%, respectively. At this condition, LCC1® was able to generate 514.5 kJ cumulative heat output in 361 s, yielding a maximum heating rate of 3.57 kW. The parametric study revealed that the absorption behaviour of A3® was more sensitive towards changes in supply pressure as well as HTF temperature compared to LCC1®. Compared to heating performance, the cooling performance of both the alloys was lower. Based on the outcomes of the experimental study, it was suggested to utilize LCC1® for decentralized hydrogen storage cum heating applications in the temperature range of 15–35 °C. 

Performance tests on Embedded Cooling Tube type Metal Hydride reactor for heating and cooling applications

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Performance tests on Embedded Cooling Tube type Metal Hydride reactor for heating and cooling applications