Abstract Conductive hydrogels have recently attracted extensive attention in the field of smart wearable electronics. Despite the current versatility of conductive hydrogels, the balance between mechanical properties (tensile properties, strength, and toughness) and electrical properties (electrical conductivity, sensitivity, and stability) still faces great challenges. Herein, a simplified method for constructing hydrophobic association hydrogels with excellent mechanical and electrical properties is proposed. The prepared conductive hydrogels exhibit high tensile properties (≈1224%), high linearity in the whole‐strain–range ( R 2 = 0.999), and a wide strain sensing range (2700%). The conductive hydrogel can realize more than 1000 cycles of sensing under 500% tensile strain. As an application demonstration, an underwater communication device is assembled in combination with polydimethylsiloxane/Triton X‐100 film coating, which successfully transmits underwater signals and provides warning of potential hazards. This study provides a new research method for developing underwater equipment with excellent mechanical properties and sensing properties. 

Flexible MXene‐Based Hydrogel Enables Wearable Human–Computer Interaction for Intelligent Underwater Communication and Sensing Rescue

Heart rate at rest and exercise may predict cardiovascular risk. Heart rate variability is a measure of variation in time between each heartbeat, representing the balance between the parasympathetic and sympathetic nervous system and may predict adverse cardiovascular events. With advances in technology and increasing commercial interest, the scope of remote monitoring health systems has expanded. In this review, we discuss the concepts behind cardiac signal generation and recording, wearable devices, pros and cons focusing on accuracy, ease of application of commercial and medical grade diagnostic devices, which showed promising results in terms of reliability and value. Incorporation of artificial intelligence and cloud based remote monitoring have been evolving to facilitate timely data processing, improve patient convenience and ensure data security.

/pdf/wearable-devices-for-remote-monitoring-of-heart-rate-and-22c2bssl.pdf

Wearable Devices for Remote Monitoring of Heart Rate and Heart Rate Variability—What We Know and What Is Coming

Electronic skin (E‐skin), especially the wearable sensors efficiently detect various stimuli attracted huge research interest owing to their potential applications in health monitoring and artificial intelligence. On the other hand, functional polymer composites possessing excellent properties such as light weight, good flexibility, and superior electrical performances, are promising candidates as building blocks for flexible electronics. Accordingly, tremendous efforts are devoted to the development of polymer composites with functional properties for E‐skin applications. Here, recent advances on the controlled fabrication of various fillers based functional polymer composites and their diverse applications in E‐skin are reviewed. In addition, contemporary studies on fabrication strategies, working mechanisms, and device performance for E‐skin based on the functional polymer composites are reviewed, including flexible pressure sensors, strain sensors, temperature sensors, energy harvesters, and transistors. Furthermore, the applications of functional composite based flexible electronics in healthcare and artificial intelligence are discussed. Finally, the existing challenges and opportunities for the functional composite materials based E‐skin are summarized.

Advanced Functional Composite Materials toward E‐Skin for Health Monitoring and Artificial Intelligence

Smart wearable systems for health monitoring are highly desired in personal wisdom medicine and telemedicine. These systems make the detecting, monitoring, and recording of biosignals portable, long-term, and comfortable. The development and optimization of wearable health-monitoring systems have focused on advanced materials and system integration, and the number of high-performance wearable systems has been gradually increasing in recent years. However, there are still many challenges in these fields, such as balancing the trade-off between flexibility/stretchability, sensing performance, and the robustness of systems. For this reason, more evolution is required to promote the development of wearable health-monitoring systems. In this regard, this review summarizes some representative achievements and recent progress of wearable systems for health monitoring. Meanwhile, a strategy overview is presented about selecting materials, integrating systems, and monitoring biosignals. The next generation of wearable systems for accurate, portable, continuous, and long-term health monitoring will offer more opportunities for disease diagnosis and treatment.

/pdf/smart-wearable-systems-for-health-monitoring-52c2lf5j.pdf

Smart Wearable Systems for Health Monitoring

Graphene and Its Derivatives: Synthesis and Application in the Electrochemical Detection of Analytes in Sweat

Soft electronic devices and sensors have shown great potential for wearable and ambulatory electrophysiologic signal monitoring applications due to their light weight, ability to conform to human skin, and improved wearing comfort, and they may replace the conventional rigid electrodes and bulky recording devices widely used nowadays in clinical settings. Herein, we report an elastomeric sponge electrode that offers greatly reduced electrode–skin contact impedance, an improved signal-to-noise ratio (SNR), and is ideally suited for long-term and motion-artifact-tolerant recording of high-quality biopotential signals. The sponge electrode utilizes a porous polydimethylsiloxane sponge made from a sacrificial template of sugar cubes, and it is subsequently coated with a poly(3,4-ethylenedioxythiophene) polystyrenesulfonate (PEDOT:PSS) conductive polymer using a simple dip-coating process. The sponge electrode contains numerous micropores that greatly increase the skin–electrode contact area and help lower the contact impedance by a factor of 5.25 or 6.7 compared to planar PEDOT:PSS electrodes or gold-standard Ag/AgCl electrodes, respectively. The lowering of contact impedance resulted in high-quality electrocardiogram (ECG) and electromyogram (EMG) recordings with improved SNR. Furthermore, the porous structure also allows the sponge electrode to hold significantly more conductive gel compared to conventional planar electrodes, thereby allowing them to be used for long recording sessions with minimal signal degradation. The conductive gel absorbed into the micropores also serves as a buffer layer to help mitigate motion artifacts, which is crucial for recording on ambulatory patients. Lastly, to demonstrate its feasibility and potential for clinical usage, we have shown that the sponge electrode can be used to monitor uterine contraction activities from a patient in labor. With its low-cost fabrication, softness, and ability to record high SNR biopotential signals, the sponge electrode is a promising platform for long-term wearable health monitoring applications.

https://pubs.acs.org/doi/pdf/10.1021/acsnano.2c04962

Stretchable Sponge Electrodes for Long-Term and Motion-Artifact-Tolerant Recording of High-Quality Electrophysiologic Signals

Soft wearable sensors are essential components for applications such as motion tracking, human-machine interface, and soft robots. However, most of the reported sensors are either specifically designed to target an individual stimulus or capable of responding to multiple stimuli (e.g., pressure and strain) but without the necessary selectivity to distinguish those stimuli. Here we report an elastomeric sponge-based sensor that can respond to and distinguish three different kinds of stimuli: pressure, strain, and temperature. The sensor utilizes a porous polydimethylsiloxane (PDMS) sponge fabricated from a sugar cube sacrificial template, which was subsequently coated with a poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) conductive polymer through a low-cost dip-coating process. Responses to different types of stimuli can be distinguished by simultaneously recording resistance and capacitance changes. Because pressure, tensile strain, and temperature change result in different trends in resistance and capacitance change, those stimuli can be clearly distinguished from each other by simultaneously measuring the resistance and capacitance of the sensor. We have also studied the effect of the pore size on the sensor performance and have found that the sponge sensor with smaller pores generally offers greater resistance change and better sensitivity. As a proof-of-concept, we have demonstrated the use of the porous sponge sensor on an artificial hand for object detection, gesture recognition, and temperature sensing applications.

https://zenodo.org/record/6390024/files/Accepted_Manuscript.pdf

A Soft Sponge Sensor for Multimodal Sensing and Distinguishing of Pressure, Strain, and Temperature.

Handwriting of perovskite optoelectronic devices on diverse substrates

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Stretchable Sponge Electrodes for Long-Term and Motion-Artifact-Tolerant Recording of High-Quality Electrophysiologic Signals

A Soft Sponge Sensor for Multimodal Sensing and Distinguishing of Pressure, Strain, and Temperature.

Handwriting of perovskite optoelectronic devices on diverse substrates