Conducting polymer hydrogels are widely used as strain sensors in light of their distinct skin‐like softness, strain sensitivity, and environmental adaptiveness in the fields of wearable devices, soft robots, and human‐machine interface. However, the mechanical and electrical properties of existing conducting polymer hydrogels, especially fatigue‐resistance and sensing robustness during long‐term application, are unsatisfactory, which severely hamper their practical utilities. Herein, a strategy to fabricate conducting polymer hydrogels with anisotropic structures and mechanics is presented through a combined freeze‐casting and salting‐out process. The as‐fabricated conducting polymer hydrogels exhibit high fatigue threshold (>300 J m−2), low Young's modulus (≈100 kPa), as well as long‐term strain sensing robustness (over 10 000 cycles). Such superior performance enables their application as strain sensors to monitor the real‐time movement of underwater robotics. The design and fabrication strategy for conducting polymer hydrogels reported in this study may open up an enticing avenue for functional soft materials in soft electronics and robotics.

Fatigue‐Resistant Conducting Polymer Hydrogels as Strain Sensor for Underwater Robotics

Transparent wood-based functional materials via a top-down approach

Wind turbine blades are often covered with ice and snow, which inevitably reduces their power generation efficiency and lifetime. Recently, a superhydrophobic surface has attracted widespread attention due to its potential values in anti-icing/deicing. However, the superhydrophobic surface can easily transition from Cassie-Baxter to Wenzel at low temperature, limiting its wide applications. Herein, inspired by the excellent water resistance and cold tolerance of Trifolium repens L. endowed by its micronano structure and low surface energy, a fresh structure was prepared by combining femtosecond laser processing technology and a boiling water treatment method. The prepared icephobic surface aluminum alloy (ISAl) mainly consists of a periodic microcrater array, nonuniform microclusters, and irregular nanosheets. This three-scale structure greatly promotes the stability of the Cassie-Baxter state. The critical Laplace pressure of ISAl is up to 1437 Pa, and the apparent water contact angle (CA) is higher than 150° at 0 °C. Those two factors contribute to its excellent anti-icing and deicing performances. The results show that the static icing delay time reaches 2577 s, and the ice adhesion strength is only 1.60 kPa. Furthermore, the anti-icing and deicing abilities of the proposed ISAl were examined under the environment of low temperature and high relative humidity to demonstrate its effectiveness. The dynamic anti-icing time of ISAl in extreme environments is up to 5 h, and ice can quickly fall with a speed of 34 r/min when it is in a horizontal rotational motion. Finally, ISAl has excellent reusability and mechanical durability, with the ice adhesion strength still being less than 6 kPa and the CA greater than 150° after 15 cycles of icing-deicing tests. The proposed structure would offer a promising strategy for the efficient anti-icing and deicing of wind turbine blades.

Trifolium repens L.-Like Periodic Micronano Structured Superhydrophobic Surface with Ultralow Ice Adhesion for Efficient Anti-Icing/Deicing.

Abstract Conductive hydrogels have recently attracted extensive attention in the field of smart wearable electronics. Despite the current versatility of conductive hydrogels, the balance between mechanical properties (tensile properties, strength, and toughness) and electrical properties (electrical conductivity, sensitivity, and stability) still faces great challenges. Herein, a simplified method for constructing hydrophobic association hydrogels with excellent mechanical and electrical properties is proposed. The prepared conductive hydrogels exhibit high tensile properties (≈1224%), high linearity in the whole‐strain–range ( R 2 = 0.999), and a wide strain sensing range (2700%). The conductive hydrogel can realize more than 1000 cycles of sensing under 500% tensile strain. As an application demonstration, an underwater communication device is assembled in combination with polydimethylsiloxane/Triton X‐100 film coating, which successfully transmits underwater signals and provides warning of potential hazards. This study provides a new research method for developing underwater equipment with excellent mechanical properties and sensing properties. 

Flexible MXene‐Based Hydrogel Enables Wearable Human–Computer Interaction for Intelligent Underwater Communication and Sensing Rescue

The application of gel wearable sensors in aquatic environments is very promising, however, the preparation of underwater gel sensors with excellent anti‐swelling properties and sensing performance remains a great challenge. In this paper, a solvent exchange strategy is proposed to fabricate an anti‐swelling gel, in which the hydrophobic segments are induced to gather and microphase separation occurs inside the gel. The prepared gel possesses excellent anti‐swelling performance (swelling ratio of 4.79%), good mechanical properties (tensile strain of 712%), high sensitivity (GF = 1.07), and high linearity (R2 = 0.998, 0 to 70% strain range). Moreover, it can achieve high stability (more than 90 days) and fatigue resistance (1000 cycles at 50% strain) as an underwater sensor. Therefore, the designed underwater gel strain sensors can be utilized for monitoring human motion information, underwater distress and smart alarms, revealing the great potential application in the field of underwater strain sensors.

Anti‐Swelling Gel Wearable Sensor Based on Solvent Exchange Strategy for Underwater Communication

Anti-swellable cellulose hydrogel for underwater sensing.

Biomass-based epoxy resin derived from resveratrol with high temperature resistance and intrinsic flame retardant properties

Reversible photo-responsive smart wood with resistant to extreme weather

The preparation, properties, functionality of a eugenol-based epoxy resin for bronze ware repairment

Real-time monitoring of human activities is of great significance for skill training and posture correction. Here, we design a cellulose derivative based electrospun nanofibrous piezoelectric mat with excellent flexibility and...

Electrospun cellulose-based nanofiber piezoelectric membrane with enhanced flexibility and pressure sensitivity

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