The different approaches in which self-assembled monolayers (SAMs) have been applied in electroanalytical chemistry are reviewed. Three principal concepts have been used and can be categorized according to the mechanism of attachment of the monolayer to the electrode. These include the formation of covalent bonds between reactive organic molecules, such as chlorosilanes, with activated surfaces, the formation of lipid and bilayer lipid membranes that self-assemble on conductive surfaces and the adsorption of functionalized alkanes, e.g., alkanethiols, on well ordered surfaces. Systems for detecting inorganic, organic and biological species are described and conclusions are drawn.

Applications of self-assembled monolayers in electroanalytical chemistry

Electrochemical studies of thallium(I) transport across gramicidin modified electrode-adsorbed phospholipid monolayers

Substrate-induced structural changes in electrode-adsorbed lipid layers: A self-consistent field theory

Electrochemical and spectroscopic studies of the mechanism of monolayer and multilayer adsorption of an insoluble surfactant at the Au(111) | electrolyte interface

Electrochemical and spectroelectrochemical characterization of lipid organization in an electric field

Initial applications of phospholipid-coated mercury electrodes to the determination of polynuclear aromatic hydrocarbons and other organic micropollutants in aqueous systems

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Initial applications of phospholipid-coated mercury electrodes to the determination of polynuclear aromatic hydrocarbons and other organic micropollutants in aqueous systems