In recent years, nanomaterials and composites have become increasingly significant as adsorbents in the removal of dyes and phenolic contaminants from wastewater. This study presents the development and application of a keratin-based graphene oxide nanocomposite, distinguished by its enhanced biocompatibility, cost-effectiveness, and strong affinity for organic compounds, making it highly effective in reducing dyes within tannery effluent. The nanocomposite was prepared via solution casting method, with dispersibility, chemical bonding, and morphology analyzed by UV–Vis spectroscopy, FTIR, and SEM, respectively. Furthermore, investigations of the influence of several factors, such as contact time, pH, and adsorbent dosage on the optimization of the process were conducted. An observation indicated a reduction of approximately 98.8 % in dye content within 20 min, achieved through the use of an adsorbent dosage of 1.5 g/L, with the solution pH maintained at 5. Subsequently, adsorption kinetics and isotherm modelling were analyzed. The results revealed that the adsorption process follows the pseudo-second-order kinetics and Freundlich isotherm models. Hence, the adsorption could be explained as chemisorption with a multilayer adsorption mechanism. Notably, a substantial reduction in parameters such as Biological Oxygen Demand (BOD) and Chemical Oxygen Demand (COD) was also achieved up to 62 % and 79 %, respectively. Therefore, the developed adsorbent could be suggested as a viable candidate for eliminating dyes from the wastewater, especially from the tannery effluent. 

Fabrication and performance analysis of keratin based-graphene oxide nanocomposite to remove dye from tannery wastewater

In recent years, there has been a growing concern to counter environmental pollution, and as a result, the development of biodegradable materials in various applications has become a major focus. This study aimed to fabricate a biodegradable composite by utilizing discarded hair keratin from beam house in leather processing along with incorporating graphene oxide (GO) to reduce pollution. The composite was prepared using a simple solution mixing method, where the amino functional group of keratin and carboxyl group of GO were covalently bonded under a redox system. Various analyses, including UV‐Vis spectroscopy, Fourier transform infrared spectroscopy (FT‐IR), Raman spectroscopy, Scanning electron microscopy (SEM), biodegradability, and oxygen gas transmittance rate (OTR), were carried out to evaluate the composite's structure and performance. The results demonstrated that GO was successfully integrated into the keratin matrix, with uniform dispersion of GO observed instead of agglomeration. The composite with the optimum ratio exhibited a 173.98% increase in tensile strength and a 33.52% decrease in elongation, as well as improved thermal and biodegradation properties compared to pure keratin. Furthermore, the composite displayed significantly better gas barrier properties (39%) than pure keratin, which can be attributed to the reduction of intermolecular gaps through the composite's strong bonding. Hence, the Keratin‐GO composite is a cost‐effective and biodegradable solution to waste materials, with potential use as a packaging material.This article is protected by copyright. All rights reserved.

Biodegradable composite from discarded hair keratin and graphene oxide with improved mechanical, thermal and barrier properties: An eco‐friendly solution to waste materials

Bio‐based waste from households and industries is a big problem for the world, however, turning it into valuable composite materials can offer a promising approach to deal with it. It involves the conversion of waste from different bio‐based sources such as cellulose waste from farming and forestry leftovers, chitin waste from seafood and mushrooms, and keratin waste from hair, nails, and feathers into natural fibers. These fibers are then effectively mixed with other materials to create composite materials having unique properties, such as high strength and stiffness, good thermal and electrical conductivity, and better barrier properties. Developing these materials is not just good for the environment because it reduces landfill waste and the reliance on non‐renewable resources, but it can also make economic sense for producers. In this review, the basic compounds of natural fibers and the development of composite materials from them are explored and discussed in detail. Furthermore, their chemical and mechanical properties are discussed and summarized. In the final section, a brief overview of the challenges and the future research needed in this fast‐evolving field is given.

Preparation of Sustainable Composite Materials from Bio‐Based Domestic and Industrial Waste: Progress, Problems, and Prospects‐ A Review

Investigating the Reinforcing Effect of Jute Fiber in a PLA & PBAT Biopolymer Blend matrix for Advanced Engineering Applications: Enhancing Sustainability with Bioresources

Utilization of GO-CS-AgNP nanocomposite for organic pollutant removal from tannery wastewater: A sustainable approach

Addressing solid waste recycling, this study aims to develop biodegradable kraft paper from buffing dust (BD) and post‐consumed jute fiber (JF). Employing a simple solution casting method with a polyurethane binder, the kraft paper was fabricated and characterized using UV–Vis spectroscopy, FTIR, XRD, SEM, TGA, OTR, biodegradability, and tensile tests. The findings revealed covalent and hydrogen bonding between BD and JF, forming a uniform surface. Notably, the composite exhibited improved thermal stability, enhanced gas barrier properties, and biodegradability compared to individual components. Furthermore, the composite also showed 57% higher tensile strength, 38% greater elongation, 20% increased hardness, and 9% higher density compared to buffing dust. Compared to jute fiber, the increases were 125%, 91%, 30%, and 19% respectively. Moreover, the composite excelled in gas barrier performance, surpassing BD and JF by a remarkable 61% and 73% increase respectively. These significant findings underscore the vast potential of the composite kraft paper as a versatile material suitable for various applications, including packaging, interior furnishing industries, and reinforcing elements in the footwear industry. By addressing waste management and promoting sustainability, this research contributes to the development of eco‐friendly materials that align with contemporary environmental concerns.
Covalent and hydrogen bonding enhance uniformity.
Biodegradable kraft paper with improved properties.
Impressive tensile strength, elongation, and hardness.
Versatile material for eco‐friendly applications.
Promotes sustainability and waste management.


Fabrication of biodegradable kraft paper from buffing dust and jute fiber: Green solutions for packaging

Pistachio shell biochar as a reinforcing filler in short Turkish hemp fiber composites: a path toward sustainable materials

The growing demand for sustainable materials is driving the adoption of microcrystalline cellulose (MCC) from renewable plant sources. This study investigated the isolation of MCC from Rosa indica petal (RIP) waste via acid hydrolysis. RIP was pretreated with alkali extraction and bleaching prior to acid hydrolysis. Chemical analysis revealed the composition of pretreated RIP was 79.56 wt.% cellulose, 9.87 wt.% hemicelluloses, and 5.69 wt.% lignin. Fourier‐transform infrared spectroscopy (FTIR) showed reduced peaks at 3332.88, 2851.95, and 1577.75 cm−1 after alkali treatment, indicating removal of hemicelluloses and lignin. X‐ray diffraction (XRD) found the crystallinity index of the isolated Rose indica petals cellulose (RIPC) MCC was 72.31%, suggesting effective purification. Thermogravimetric analysis (TGA) revealed RIPC MCC had a decomposition temperature of 296.65°C, superior to raw RIP at 211.25°C. In addition, atomic force microscopy (AFM) and scanning electron microscopy (SEM) showed RIPC MCC had fibrous morphology with fiber diameters ranging from 16.2–22.4 nm. In summary, RIPC MCC with high purity, crystallinity and thermal stability was successfully isolated from RIP waste via acid hydrolysis. The high performance of RIPC MCC demonstrates the potential of RIP leftovers as a renewable source for MCC production. RIPC MCC could serve as a promising reinforcement filler in nanocomposites due to its advantageous properties.

Physicochemical characterization of novel biomass‐based microcrystalline cellulose derived from agro‐industrial residues of Rosa indica petals

Taguchi fuzzy multi-response optimization of process parameters in compression molding of natural hybrid composite

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