Science and technologies based on terahertz frequency electromagnetic radiation (100 GHz–30 THz) have developed rapidly over the last 30 years. For most of the 20th Century, terahertz radiation, then referred to as sub-millimeter wave or far-infrared radiation, was mainly utilized by astronomers and some spectroscopists. Following the development of laser based terahertz time-domain spectroscopy in the 1980s and 1990s the field of THz science and technology expanded rapidly, to the extent that it now touches many areas from fundamental science to 'real world' applications. For example THz radiation is being used to optimize materials for new solar cells, and may also be a key technology for the next generation of airport security scanners. While the field was emerging it was possible to keep track of all new developments, however now the field has grown so much that it is increasingly difficult to follow the diverse range of new discoveries and applications that are appearing. At this point in time, when the field of THz science and technology is moving from an emerging to a more established and interdisciplinary field, it is apt to present a roadmap to help identify the breadth and future directions of the field. The aim of this roadmap is to present a snapshot of the present state of THz science and technology in 2017, and provide an opinion on the challenges and opportunities that the future holds. To be able to achieve this aim, we have invited a group of international experts to write 18 sections that cover most of the key areas of THz science and technology. We hope that The 2017 Roadmap on THz science and technology will prove to be a useful resource by providing a wide ranging introduction to the capabilities of THz radiation for those outside or just entering the field as well as providing perspective and breadth for those who are well established. We also feel that this review should serve as a useful guide for government and funding agencies.

https://iopscience.iop.org/article/10.1088/1361-6463/50/4/043001/pdf

The 2017 terahertz science and technology roadmap

Recent research and development has been incredibly successful at advancing the capabilities for vacuum electronic device (VED) sources of powerful terahertz (THz) and near-THz coherent radiation, both CW or average and pulsed. Currently, the VED source portfolio covers over 12 orders of magnitude in power (mW-to-GW) and two orders of magnitude in frequency (from ; 10 THz). Further advances are still possible and anticipated. They will be enabled by improved understanding of fundamental beam-wave interactions, electromagnetic mode competition and mode control, along with research and development of new materials, fabrication methods, cathodes, electron beam alignment and focusing, magnet technologies, THz metrology and advanced, broadband output radiation coupling techniques.

Vacuum Electronic High Power Terahertz Sources

Within the last several years, the field of terahertz science and technology has changed dramatically. Many new advances in the technology for generation, manipulation, and detection of terahertz radiation have revolutionized the field. Much of this interest has been inspired by the promise of valuable new applications for terahertz imaging and sensing. Among a long list of proposed uses, one finds compelling needs such as security screening and quality control, as well as whimsical notions such as counting the almonds in a bar of chocolate. This list has grown in parallel with the development of new technologies and new paradigms for imaging and sensing. Many of these proposed applications exploit the unique capabilities of terahertz radiation to penetrate common packaging materials and provide spectroscopic information about the materials within. Several of the techniques used for terahertz imaging have been borrowed from other, more well established fields such as x-ray computed tomography and synthetic aperture radar. Others have been developed exclusively for the terahertz field, and have no analogies in other portions of the spectrum. This review provides a comprehensive description of the various techniques which have been employed for terahertz image formation, as well as discussing numerous examples which illustrate the many exciting potential uses for these emerging technologies.

https://iopscience.iop.org/article/10.1088/0034-4885/70/8/R02/pdf

Imaging with terahertz radiation

The 2016 terahertz science and technology roadmap

Intersystem crossing (ISC), formally forbidden within nonrelativistic quantum theory, is the mechanism by which a molecule changes its spin state. It plays an important role in the excited state decay dynamics of many molecular systems and not just those containing heavy elements. In the simplest case, ISC is driven by direct spin–orbit coupling between two states of different multiplicities. This coupling is usually assumed to remain unchanged by vibrational motion. It is also often presumed that spin-allowed radiationless transitions, i.e. internal conversion, and the nonadiabatic coupling that drives them, can be considered separately from ISC and spin–orbit coupling owing to the vastly different time scales upon which these processes are assumed to occur. However, these assumptions are too restrictive. Indeed, the strong mixing brought about by the simultaneous presence of nonadiabatic and spin–orbit coupling means that often the spin, electronic, and vibrational dynamics cannot be described independe...

Spin-Vibronic Mechanism for Intersystem Crossing

Terahertz scanning near-field infrared microscopy below 1 THz is demonstrated at an electron storage ring using coherent synchrotron radiation. Spatial resolution below the diffraction limit down to about λ/40 at 2 cm−1 is derived from the transmittance spectra of a conical aperture probe. The potential of the technique is exemplified by imaging wet biological samples. Strongly absorbing living leaves have been imaged in transmittance with a spatial resolution of 130 μm at about 12 cm−1. The THz near-field images reveal distinct structural differences in the mesophytic and xerophytic leaves investigated.

THz near-field imaging employing synchrotron radiation

We present first ideas of a scheme to develop BESSY II into a variable electron pulse length storage ring. The final goal is, to fill BESSY II with short bunches of 1.5 ps length (rms) and long bunches of 15 ps length simultaneously in the presently applied user optics. All insertion devices are operated as usual, i.e. the helical undulators and 7 T-field insertions. Long bunches of 1.5 mA current per bunch, twice the value of the present user optics, are filled in each second bucket. The other buckets can be filled with short bunches of up to 0.8 mA. The lower current value is required to avoid increase in the bunch length and bunch energy spread, predicted by scaling laws. The total current is e.g. limited by the HOM damping capabilities of the sccavities and the machine impedances. This scheme is achievable with recent developments in sc-rf cavity technology driven by requirements of high current cw applications like for the energy recovering linacs (ERLs). These developments seem to make it feasible to install high gradient HOM damped multi-cell cavities in electron storage rings. With an appropriate choice of the cavity resonance frequencies a beating of the effective longitudinal focusing voltage at the stable fixed points can be introduced and leads to different zero current bunch lengths. Basic parameters of this scheme are presented.

Simultaneous long and short electron bunches in the bessy ii storage ring

This presentation covers analytical models that describe the interaction of a relativistic particle beam with the magnetic field of undulators Analytic approximations to the Hamilton-Jacobi equation yield generating functions useful for particle tracking and, therefore, efficient simulation Analytic expressions for kick maps of APPLE II undulators are presented as well Passive and active shimming schemes including magic fingers and current sheets are also modelled Applications at BESSY II are discussed which ensure efficient injection during top-up to satisfy machine protection and radiation safety requirements

Symplectic tracking and compensation of dynamic field integrals in complex undulator structures

At BESSY bursts of coherent synchrotron radiation around 20 cm/sup -1/ have been observed above a certain threshold current. The repetition rate of these bursts depends on the beam current and the thresholds vary strongly with the bunch length. Observed thresholds are in agreement with the theory of beam instability and microbunching due to coherent synchrotron radiation (CSR).

Coherent emission of synchrotron radiation and longitudinal instabilities

Significant progress has been made in the last few years in short-bunch operation of third-generation synchrotron light sources, achieved by “lowα” optics for storage rings [1–4]. The term α is a machine optics parameter describing the particle orbit length L as a function of the particle momentum p, L = L0(1 + α(p − p0)/p0), with respect to the nominal values indicated by the index “0”. The “zero current” bunch length σ is then proportional to . Included here is the rf-voltage temporal gradient, V′ = dV/dt, which additionally influences the bunch length and will be required further. Thus, lowering α leads to a reduced bunch length all around the ring and radiation of the short bunches is supplied to all beamlines. These short bunches produce short X-ray pulses of equal length suitable for time-resolved measurements. Simultaneously, the short electron pulses emit intense, coherent THz radiation.

Low-α Operation of BESSY II and Future Plans for an Alternating Bunch Length Scheme BESSYVSR

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