Carbon dioxide capture-related gas adsorption and separation in metal-organic frameworks

Post-combustion CO2 capture from the flue gas is one of the key technology options to reduce greenhouse gases, because this can be potentially retrofitted to the existing fleet of coal-fired power stations. Adsorption processes using solid sorbents capable of capturing CO2 from flue gas streams have shown many potential advantages, compared to other conventional CO2 capture using aqueous amine solvents. In view of this, in the past few years, several research groups have been involved in the development of new solid sorbents for CO2 capture from flue gas with superior performance and desired economics. A variety of promising sorbents such as activated carbonaceous materials, microporous/mesoporous silica or zeolites, carbonates, and polymeric resins loaded with or without nitrogen functionality for the removal of CO2 from the flue gas streams have been reviewed. Different methods of impregnating functional groups, including grafting techniques and modifying the support materials, have been discussed to en...

Post-Combustion CO2 Capture Using Solid Sorbents: A Review

Rapid synthesis of zeolitic imidazolate framework-8 (ZIF-8) nanocrystals in an aqueous system

Metal-organic framework (MOF) materials, which are constructed from metal ions or metal ion clusters and bridging organic linkers, exhibit regular crystalline lattices with relatively well-defined pore structures and interesting properties. As a new class of porous solid materials, MOFs are attractive for a variety of industrial applications including separation membranes - a rapidly developing research area. Many reports have discussed the synthesis and applications of MOFs and MOF thin films, but relatively few have addressed MOF membranes. This critical review provides an overview of the diverse MOF membranes that have been prepared, beginning with a brief introduction to the current techniques for the fabrication of MOF membranes. Gas and liquid separation applications with different MOF membranes are also included (175 references).

Metal–organic framework membranes: from synthesis to separation application

This Review details the structural and chemical features of state-of-the-art metal–organic frameworks for their application in the entire carbon cycle of capturing, purifying and transforming CO 2 into valuable products.

The chemistry of metal–organic frameworks for CO 2 capture, regeneration and conversion

Synthesis and characterization of ZIF-69 membranes and separation for CO2/CO mixture

Preparation of metal oxide/zeolite core–shell nanostructures

Synthesis of highly c-oriented AFI membranes by epitaxial growth

The adsorption properties of an aluminophosphate molecular sieve, SAPO-5, were measured for a number of gases and vapors, including N2, water, isopropanol, and xylenes. The data showed that SAPO-5 is quite hydrophobic and has a strong selectivity of o-xylene over its isomers m- and p-xylene.

Adsorption Properties of the SAPO-5 Molecular Sieve

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Synthesis and characterization of ZIF-69 membranes and separation for CO2/CO mixture

Preparation of metal oxide/zeolite core–shell nanostructures

Synthesis of highly c-oriented AFI membranes by epitaxial growth

Adsorption Properties of the SAPO-5 Molecular Sieve