Laboratory tests, field application and carbon footprint assessment of cement-stabilized pure coal solid wastes as pavement base materials

Utilization of raw coal gangue as coarse aggregates in pavement concrete

A systematic review exploring the utilization of coal mining and processing wastes as secondary aggregate in sub-base and base layers of pavement

Extracting valuable elements from coal gangue is an important method for the utilization of coal gangue. In order to obtain the suitable technological conditions and the acid leaching kinetic model of leaching aluminum and iron ions from high-iron and low-aluminum coal gangue, the effects of calcination temperature, calcination time, and acid types on the leaching results of aluminum and iron ions are studied. The results show that when the gangue is calcined at 675 °C for 1 h, then the calcined gangue powder is leached by 6 mol/L hydrochloric acid at 93 °C for 4 h, the leaching ratio of iron ions is more than 90%, and that of aluminum ions is more than 60%. Furthermore, the acid leaching kinetic equations at 30 °C, 50 °C, 70 °C, and 90 °C are studied by three kinetic models, and the apparent activation energies of the reactions are calculated by the Arrhenius formula. The results show that the leaching behavior of aluminum and iron ions conformed to the “mixing control” model equation: “(1 − x)−1/3 − 1 + 1/3ln(1 − x) = kt + b”. The apparent activation energies of aluminum and iron ions are 55.5 kJ/mol and 55.8 kJ/mol, respectively. All these indicate that the acid leaching process is controlled by the “mixing control”.

https://www.mdpi.com/2075-163X/12/2/215/pdf?version=1644480224

Extraction of Aluminum and Iron Ions from Coal Gangue by Acid Leaching and Kinetic Analyses

Poly aluminum-ferric Chloride (PAFC) is a new type of high efficiency coagulant. In this study, high iron type gangue is used as a main raw material. It is calcined at 675 °C for 1 h and 3% CaF2 is added to the calcined powder and reacted with 20% hydrochloric acid at 93 °C for 4 h. The leaching ratio of aluminum ions is 90% and that of iron ions is 91%. After Fe2+ ions are oxidized in the filtrate, CaCO3 is used to adjust the pH of the filtrate to 0.7. The microwave power is adjusted to 80 W and the filtrate is radiated for 5 min. After being aged for 24 h, PAFC product is obtained. The prepared PAFC is used to treat mine water and compared with the results of PAC and PAF, the turbidity removal ratio of PAFC is 99.6%, which is greater than 96.4% of PAC and 93.7% of PAF. PAFC is a mixture with different degrees of polymerization. It demonstrates that extracting aluminum and iron ions from high iron content gangue to prepare PAFC by microwave is efficient and feasible.

/pdf/preparation-of-poly-aluminum-ferric-chloride-pafc-coagulant-30o0cgts.pdf

Preparation of Poly Aluminum-Ferric Chloride (PAFC) Coagulant by Extracting Aluminum and Iron Ions from High Iron Content Coal Gangue

The research into the road performance of coal gangue is of great significance for the consumption of coal gangue and reducing pollution. In this paper, the coal gangues were prepared by separation and crushing processes, and their gradations were also optimized. Aiming to identify the possible problems of coal gangue as a pavement base, an unconfined compressive strength test, a splitting test, a freeze–thaw test, and a drying shrinkage test of cement stabilized gangue with varying cement amounts were carried out, and the test results were compared and analyzed. The test results showed that the maximum dry density and optimum moisture content (OMC) of the optimized cement stabilized gangue and cement stabilized macadam increased with cement content. The maximum dry density and OMC of cement stabilized macadam were larger than that of cement stabilized gangue with the same cement content. The optimized 7-day unconfined compressive strength of cement stabilized gangue can meet the requirements for a secondary and lower highway base and subbase. The OMC and cement content are the critical factors affecting the compressive strength loss rate of cement stabilized gangue after freeze–thaw cycles. The smaller the OMC of cement stabilized gangue and the larger the cement content, the lower the compressive strength loss rate. With an increase in cement content, the drying shrinkage strain of cement stabilized gangue increased. The results show that a cement content of 4% is optimal for the cement stabilized coal gangue, which can be used for the light traffic base and heavy traffic subbase of class II and below highways. It provides a basis, guide, and reference for the application of coal gangue materials in a high-grade highway base.

An Experimental Study of the Road Performance of Cement Stabilized Coal Gangue

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An Experimental Study of the Road Performance of Cement Stabilized Coal Gangue