Holography has been identified as a vital platform for three-dimensional displays, optical encryption, microscopy and artificial intelligence through different physical dimensions. However, unlike the wavelength and polarization divisions, orbital angular momentum (OAM) of light, despite its helical wavefront being an independent physical dimension, has not been implemented as an information carrier for holography due to the lack of helical mode index selectivity in the Bragg diffraction formula. Here, we demonstrate OAM holography by discovering strong OAM selectivity in the spatial-frequency domain without a theoretical helical mode index limit. As such, OAM holography allows the multiplexing of a wide range of OAM-dependent holographic images with a helical mode index spanning from −50 to 50, leading to a 10 bit OAM-encoded hologram for high-security optical encryption. Our results showing up to 210 OAM-dependent distinctive holographic images mark a new path to achieving ultrahigh-capacity holographic information systems harnessing the previously inaccessible OAM division. The orbital angular momentum degree of freedom is used to demonstrate 10 bit holographic images with a helical mode index spanning from −50 to 50.

Orbital angular momentum holography for high-security encryption

All forms of energy follow the law of conservation of energy, by which they can be neither created nor destroyed. Light-to-heat conversion as a traditional yet constantly evolving means of converting light into thermal energy has been of enduring appeal to researchers and the public. With the continuous development of advanced nanotechnologies, a variety of photothermal nanomaterials have been endowed with excellent light harvesting and photothermal conversion capabilities for exploring fascinating and prospective applications. Herein we review the latest progresses on photothermal nanomaterials, with a focus on their underlying mechanisms as powerful light-to-heat converters. We present an extensive catalogue of nanostructured photothermal materials, including metallic/semiconductor structures, carbon materials, organic polymers, and two-dimensional materials. The proper material selection and rational structural design for improving the photothermal performance are then discussed. We also provide a representative overview of the latest techniques for probing photothermally generated heat at the nanoscale. We finally review the recent significant developments of photothermal applications and give a brief outlook on the current challenges and future directions of photothermal nanomaterials.

https://pubs.acs.org/doi/pdf/10.1021/acs.chemrev.3c00159

Photothermal Nanomaterials: A Powerful Light-to-Heat Converter

Digital optical holograms can achieve nanometre-scale resolution as a result of recent advances in metasurface technologies. This has raised hopes for applications in data encryption, data storage, information processing and displays. However, the hologram bandwidth has remained too low for any practical use. To overcome this limitation, information can be stored in the orbital angular momentum of light, as this degree of freedom has an unbounded set of orthogonal helical modes that could function as information channels. Thus far, orbital angular momentum holography has been achieved using phase-only metasurfaces, which, however, are marred by channel crosstalk. As a result, multiplex information from only four channels has been demonstrated. Here, we demonstrate an orbital angular momentum holography technology that is capable of multiplexing up to 200 independent orbital angular momentum channels. This has been achieved by designing a complex-amplitude metasurface in momentum space capable of complete and independent amplitude and phase manipulation. Information was then extracted by Fourier transform using different orbital angular momentum modes of light, allowing lensless reconstruction and holographic videos to be displayed. Our metasurface can be three-dimensionally printed in a polymer matrix on SiO2 for large-area fabrication.

/pdf/complex-amplitude-metasurface-based-orbital-angular-momentum-1t1lmm8j59.pdf

Complex-amplitude metasurface-based orbital angular momentum holography in momentum space.

The absorption of light by plasmonic nanostructures and their associated temperature increase are exquisitely sensitive to the shape and composition of the structure and to the wavelength of light. Therefore, much effort is put into synthesizing novel nanostructures for optimized interaction with the incident light. The successful synthesis and characterization of high quality and biocompatible plasmonic colloidal nanoparticles has fostered numerous and expanding applications, especially in biomedical contexts, where such particles are highly promising for general drug delivery and for tomorrow's cancer treatment. We review the thermoplasmonic properties of the most commonly used plasmonic nanoparticles, including solid or composite metallic nanoparticles of various dimensions and geometries. Common methods for synthesizing plasmonic particles are presented with the overall goal of providing the reader with a guide for designing or choosing nanostructures with optimal thermoplasmonic properties for a given application. Finally, the biocompatibility and biological tolerance of structures are critically discussed along with novel applications of plasmonic nanoparticles in the life sciences.

Plasmonic Heating of Nanostructures.

Acoustic tweezers use sound radiation forces to manipulate matter without contact. They provide unique characteristics compared with the more established optical tweezers, such as higher trapping forces per unit input power and the ability to manipulate objects from the micrometer to the centimeter scale. They also enable the trapping of a wide range of sample materials in various media. A dramatic advancement in optical tweezers was the development of holographic optical tweezers (HOT) which enabled the independent manipulation of multiple particles leading to applications such as the assembly of 3D microstructures and the probing of soft matter. Now, 20 years after the development of HOT, we present the realization of holographic acoustic tweezers (HAT). We experimentally demonstrate a 40-kHz airborne HAT system implemented using two 256-emitter phased arrays and manipulate individually up to 25 millimetric particles simultaneously. We show that the maximum trapping forces are achieved once the emitting array satisfies Nyquist sampling and an emission phase discretization below π/8 radians. When considered on the scale of a wavelength, HAT provides similar manipulation capabilities as HOT while retaining its unique characteristics. The examples shown here suggest the future use of HAT for novel forms of displays in which the objects are made of physical levitating voxels, assembly processes in the micrometer and millimetric scale, as well as positioning and orientation of multiple objects which could lead to biomedical applications.

/pdf/holographic-acoustic-tweezers-4y4s40k9bo.pdf

Holographic acoustic tweezers

Photophoretic optical trapping of cellulose particles and persistence of vision are used to produce real-space volumetric images that can be viewed from all angles, in geometries unachievable by holograms and light-field technologies. Three-dimensional moving images have long been the stuff of science fiction. In reality, the appearance of three dimensions is usually approximated by manipulating light, but such approaches have limitations such as narrow viewing angles and the need for special viewing headwear. Daniel Smalley and colleagues offer a solution in which a three-dimensional object can be represented in real space, viewed from any angle, and even coexist with—and wrap around—solid objects that occupy the same physical volume. A near-invisible light field traps and moves a small particle through a volume of space. As the particle moves, it is illuminated using red, green and blue laser light, producing an arbitrarily coloured point-source that maps out the surface of the object to be imaged. If the particle scanning is fast enough, persistence of vision, which results from the slower 'refresh rate' of the human eye, gives the appearance of a solid three-dimensional surface. At even faster scanning rates, the imaged object can appear to move. Free-space volumetric displays, or displays that create luminous image points in space, are the technology that most closely resembles the three-dimensional displays of popular fiction1. Such displays are capable of producing images in ‘thin air’ that are visible from almost any direction and are not subject to clipping. Clipping restricts the utility of all three-dimensional displays that modulate light at a two-dimensional surface with an edge boundary; these include holographic displays, nanophotonic arrays, plasmonic displays, lenticular or lenslet displays and all technologies in which the light scattering surface and the image point are physically separate. Here we present a free-space volumetric display based on photophoretic optical trapping2 that produces full-colour graphics in free space with ten-micrometre image points using persistence of vision. This display works by first isolating a cellulose particle in a photophoretic trap created by spherical and astigmatic aberrations. The trap and particle are then scanned through a display volume while being illuminated with red, green and blue light. The result is a three-dimensional image in free space with a large colour gamut, fine detail and low apparent speckle. This platform, named the Optical Trap Display, is capable of producing image geometries that are currently unobtainable with holographic and light-field technologies, such as long-throw projections, tall sandtables and ‘wrap-around’ displays1.

A photophoretic-trap volumetric display

In an effort to create a full-color holovideo display, a wavelength-multiplexing LiNbO 3 crystal is designed. Fabrication parameters are presented. Results of tests and measurements are presented, as well as the procedures used to obtain them. By matching the bandwidth of the LiNbO 3 to that of current GPUs, the display is able to efficiently process large amounts of data.

Design and fabrication of a color multiplexing LiNbO 3 device

In this presentation we report improvements to the supporting geometry of the low-cost MIT/BYU mark IV holographic video monitor and invite broader participation in this research effort by providing design equations and prototyping data.

Progress on a low-cost holographic video monitor

This paper presents an optical apparatus for characterizing frequency multiplexing of color in leaky mode, anisotropic waveguide modulators. This type of characterization is particularly useful for informing the design of full color holographic video displays. The primary function of the apparatus is to map the frequency response and angular overlap of red, green, and blue outputs. The apparatus also allows measurements of other parameters such as scan center frequency, optical and RF bandwidth, and scan linearity.

Frequency division color characterization apparatus for anisotropic leaky mode light modulators.

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A photophoretic-trap volumetric display

Design and fabrication of a color multiplexing LiNbO 3 device

Progress on a low-cost holographic video monitor

Frequency division color characterization apparatus for anisotropic leaky mode light modulators.